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Record W2766403881 · doi:10.1021/acs.est.7b02231

Low Permeability Zone Remediation via Oxidant Delivered by Electrokinetics and Activated by Electrical Resistance Heating: Proof of Concept

2017· article· en· W2766403881 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnvironmental Science & Technology · 2017
Typearticle
Languageen
FieldEngineering
TopicElectrokinetic Soil Remediation Techniques
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsElectrokinetic phenomenaEnvironmental remediationPermeability (electromagnetism)ChemistryContaminationBiochemistryBiologyEcologyMembrane

Abstract

fetched live from OpenAlex

This study proposes and proves (in concept) a novel approach of combining electrokinetic (EK)-assisted delivery of an oxidant, persulfate (PS), and low temperature electrical resistivity heating (ERH), to activate PS, to achieve remediation of contaminated, low permeability soil. This unique combination is able to overcome existing challenges in remediating low permeability materials, particularly associated with delivering remediants. A further benefit of the approach is the use of the same electrodes for both EK and ERH phases. Experiments were conducted in a laboratory-scale sand tank packed with silt and aqueous tetrachloroethene (PCE) and bracketed on each side by an electrode. EK first delivered unactivated PS throughout the silt. ERH then generated and sustained the target temperature to activate the PS. As a result, PCE concentrations decreased to below detection limit in the silt in a few weeks. Moreover, it was found that activating PS at ∼36 °C eliminated more PCE than activating it at >41 °C. It is expected this results from the reactive SO 4 •– radical being generated more slowly, which ensures more complete reaction with the contaminant. The novel application of EK-assisted PS delivery followed by low temperature ERH appears to be a viable strategy for low permeability contaminated soil remediation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.023
Threshold uncertainty score0.755

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.002
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.197
Teacher spread0.194 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it