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Record W2781334612 · doi:10.1107/s2053273317087022

Lattice location of Ta and Ti in doped Nb<sub>3</sub>Sn

2017· article· en· W2781334612 on OpenAlexfundno aff
Steve M. Heald, C. Tarantini, Peter J. Lee, Michael P. Brown, D. C. Larbalestier

Bibliographic record

VenueActa Crystallographica Section A Foundations and Advances · 2017
Typearticle
Languageen
FieldEngineering
TopicSuperconducting Materials and Applications
Canadian institutionsnot available
FundersArgonne National LaboratoryHigh Magnetic Field Laboratory, Chinese Academy of SciencesCanadian Light SourceNational High Magnetic Field LaboratoryHigh Energy PhysicsU.S. Department of EnergyDivision of Materials ResearchOffice of ScienceNational Science Foundation
KeywordsDopingMaterials scienceLattice (music)NiobiumCrystallographyCondensed matter physicsMetallurgyChemistryPhysicsOptoelectronics

Abstract

fetched live from OpenAlex

There has been renewed interest in Nb3Sn superconductor for its proposed application in the new fusion test reactor, ITER, and for next generation accelerators such as the LHC upgrade. Due to its brittle nature, an effective way to produce thin filaments of Nb3Sn in a wire is by an internal tin Restacked-Rod-Process (RRP) where each filament is made of Cu-cladded Nb (or Nb-Ti or Nb-Ta) rods restacked around a Sn core in a Cu-cladded Nb tube acting as diffusion barrier. During the heat treatment Nb and Sn react forming a continuous layer of Nb3Sn. It has been known for some time that the addition of small amounts of Ti and Ta can improve the superconducting in-field properties of the final wires. Initial measurements on Nb3Sn ribbons using electron channeling and EXAFS indicated that these dopants are primarily located at the Nb lattice sites. However, more recent studies suggest that Ti could be occupying the Sn sites. This motivated a new set of EXAFS measurements on modern wires similar to those proposed for the new applications. EXAFS is a sensitive method for looking at the lattice locations of the dopants since it looks directly at their near neighbors, and the two lattice sites have distinctly different local environments. Four different samples were measured, two with Ti doping, one with Ta doping and one with both Ta and Ti doping. In all cases the Ti and Ta were found to be primarily in the Nb sites. For the three Ti cases there was no indication of any Ti in the Sn sites. For the Ta data, the EXAFS indicated that there was partial occupancy into the Sn sites with about 18% of the Ta in the Sn site for the Ta only sample, and 34% in the co-doped sample. The implications of this result will be discussed.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.921
Threshold uncertainty score0.391

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.250
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2017
Admission routes1
Has abstractyes

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