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Record W2800097296 · doi:10.1002/cjce.23239

Study of the coke distribution in MTO fluidized bed reactor with MP‐PIC approach

2018· article· en· W2800097296 on OpenAlexvenueno aff
Xiaoshuai Yuan, Hua Li, Mao Ye, Zhongmin Liu

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2018
Typearticle
Languageen
FieldEngineering
TopicGranular flow and fluidized beds
Canadian institutionsnot available
FundersDalian Institute of Chemical PhysicsNational Natural Science Foundation of China
KeywordsCokeResidence time distributionResidence time (fluid dynamics)CatalysisFluidized bedProduct distributionChemistryChemical engineeringWaste managementMineralogyOrganic chemistryEngineering

Abstract

fetched live from OpenAlex

Abstract The methanol to olefins (MTO) process has received considerable interest due to its importance in transforming abundant resources such as coal, natural gas, and biomass to widely‐demanded light olefins. In the MTO process, the coke deposited on the catalyst governs the catalyst activity and product selectivity, and thus is critical to the reaction behaviour. In the industrial processes, the residence time and coke content of catalyst particles in the reactor show a certain distribution due to the continuous outflow of spent catalyst and inflow of regenerated catalyst, which need further attention. The multi‐phase particle‐in‐cell (MP‐PIC) approach was used in the current work to simulate the catalyst residence time and coke content distribution. The effect of gas‐solid flow patterns, reactor structure, and average catalyst residence time on the residence time and coke content distribution was investigated. It was found that at high superficial velocities, the coke content distributions obtained with the MP‐PIC method are consistent with the distribution deduced from the ideally mixed flow assumption of catalyst particles. The results suggested that it is possible to simulate large‐scale MTO reactors by use of the coke distribution. In particular, by incorporating an initial coke distribution, the time needed to reach steady state in the MTO reactor simulations could be greatly reduced.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score0.328

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.173
Teacher spread0.165 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations25
Published2018
Admission routes1
Has abstractyes

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