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Record W2900699442 · doi:10.15278/isms.2018.wh10

FIRST HIGH RESOLUTION IR SPECTRA OF 2-D1-PROPANE. THE ν9 (A1) B-TYPE BAND NEAR 367.2389 cm−1.

2018· article· en· W2900699442 on OpenAlexaff
S. J. Daunt, Brant Billinghurst, Jean‐Marie Flaud, Walter J. Lafferty, Robert Grzywacz

Bibliographic record

VenueProceedings of the 73rd International Symposium on Molecular Spectroscopy · 2018
Typearticle
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsCanadian Light Source (Canada)Canadiana.org
Fundersnot available
KeywordsSpectral lineIsotopologueHigh resolutionPropaneResolution (logic)Infrared spectroscopyPhysicsChemistryAnalytical Chemistry (journal)Atomic physicsMaterials scienceGeology

Abstract

fetched live from OpenAlex

\\begin{wrapfigure}{r}{0pt}\n\n\\includegraphics[scale=0.25]{B0157.4b.water-cntm4.eps}\n\n\\end{wrapfigure} \n\nWater is the strongest greenhouse gas in the Earth atmosphere, which plays a critical role in the energy balance of the earth atmosphere. It has long been observed particularly in the far-infrared that there is significant longwave continuum absorption due to water vapor (dimers or multimers), not attributable to the Lorentz line contribution within 25 cm$^{-1}$ from the line center for individual water vapor lines. The MT\\_CKD model offers the water vapor continuum predictions, which are to be validated by a laboratory study in the far infrared. In order to directly measure this water vapor continuum absorption, we have obtained a series of spectra of water vapor broadened by Self, N$_2$, and O$_2$ in the 50 – 500 cm$^{-1}$ (200 – 20 $\\mu$m) at temperatures between 251 and 296 K. For this, we used a coolable White cell system (whose optics are optimized for the far-infrared spectrometry) with passive temperature control, configured to the Fourier transform spectrometer, Bruker IFS-125HR at the Jet Propulsion Laboratory (JPL). \n\nWe have been analyzing the spectra to make direct measurement of the far-infrared water continuum in two steps; (1) we obtained their transmission spectra by ratioing the sample spectrum to their corresponding background spectrum, (2) we obtained the continuum part of the transmission by dividing the measured spectrum by a synthetic spectrum of the resonant lines calculated using the HITRAN database. As shown in Figure 1, it has revealed the underlying water-water, water-O$_2$, and water-N$_2$ continua in the temperature range, depending on the spectrum type. The preliminary results from this on-going analysis are presented along with their comparison with the MT\\_CKD (ver.3.5) model predictions. Temperature dependence of the water vapor continuum will be discussed as part of future work.\\footnote{Government sponsorship acknowledged}.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.113
Threshold uncertainty score0.943

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0020.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.242
Teacher spread0.235 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2018
Admission routes1
Has abstractyes

Explore more

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