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Record W2901624631 · doi:10.15278/isms.2018.ti08

DEVELOPMENT OF A HYBRID LASER-MASS SPECTROMETER WITH TWO INSTRUMENT ARMS: IRMPD AND HENDI COLD ION SPECTROSCOPIC EXPERIMENTS

2018· article· en· W2901624631 on OpenAlexaff
Yunjie Xu, Wolfgang Jäger, Haolu Wang, Zhihao Chen, Fan Xie, Joseph Cheramy, Matthias Heger

Bibliographic record

VenueProceedings of the 73rd International Symposium on Molecular Spectroscopy · 2018
Typearticle
Languageen
FieldEngineering
TopicLaser Design and Applications
Canadian institutionsUniversity of Alberta
Fundersnot available
KeywordsInfrared multiphoton dissociationMass spectrometryIonSpectrometerLaserMaterials scienceOpticsPhysics

Abstract

fetched live from OpenAlex

The [7.7] \\textit{Y} $^{2}\\Sigma^{+}$ - \\textit{X} $^{2}\\Pi_{\\textit{i}}$ transition of CuO was observed in emission from a Cu hollow cathode recorded with the FT-spectrometer associated with the McMath-Pierce Solar Telescope at Kitt Peak in 1994. In 1996, a rotational analysis of the (0,0) band of the \\textit{Y} - \\textit{X} transition was reported by O’Brien \\textit{et al}. In a recent analysis of the (0,0) and (1,1) bands of the [16.4] \\textit{A} $^{2}\\Sigma^{-}$ - \\textit{X} $^{2}\\Pi_{\\textit{i}}$ transition of CuO performed by the authors, improved centrifugal distortion constants for the \\textit{X} $^{2}\\Pi_{\\textit{i}}$ state were obtained. Line positions from the millimeter wave spectrum of CuO reported by Steimle \\textit{et al}. were successfully incorporated into the fit of the \\textit{A} – \\textit{X} transition, however, a fit including the line positions of the \\textit{Y} - \\textit{X} transition reported by O’Brien \\textit{et al}. showed small, yet significant, deviations in the residuals of the fit. In this study, the FTS data from 1994 was accessed from the FTP archive available from the National Solar Observatory website to investigate these deviations. The calibration of the data was verified to $\\pm$0.001 \\wn using Ne reference lines from Sansonetti \\textit{et al}. Using PGOPHER simulations and the improved rotational constants for the \\textit{X} $^{2}\\Pi_{\\textit{i}}$ ground state, over 1000 additional line positions belonging to the (0,0) band of the \\textit{Y} - \\textit{X} transition were identified in the FTS data. Several previously unidentified vibrational bands were also observed and rotationally analyzed using PGOPHER, specifically the (2,0), (2,1), (2,2), (2,3), (1,0), (1,1), (1,2), (1,3), (0,0), (0,1), and (0,2) bands. A comprehensive fit of the data containing more than 10,000 line positions has been conducted using PGOPHER. The fit successfully incorporated the millimeter wave data for the \\textit{X} $^{2}\\Pi_{\\textit{i}}$ state from Steimle \\textit{et al}. and the intracavity laser absorption data for the \\textit{A} - \\textit{X} state from the authors. Results of this analysis will be presented.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: Methods
Teacher disagreement score0.007
Threshold uncertainty score0.024

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0020.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0010.001
Scholarly communication0.0010.002
Open science0.0040.002
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0070.003

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.230
Teacher spread0.223 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations0
Published2018
Admission routes1
Has abstractyes

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