MétaCan
Menu
Back to cohort
Record W2911375172 · doi:10.1002/admi.201801895

An In Situ Procedure for the Preparation of Zeolitic Imidazolate Framework‐8 Polyacrylamide Hydrogel for Adsorption of Aqueous Pollutants

2019· article· en· W2911375172 on OpenAlexafffund
Omar Maan, Ping Song, Ningxin Chen, Qingye Lu

Bibliographic record

VenueAdvanced Materials Interfaces · 2019
Typearticle
Languageen
FieldChemistry
TopicMetal-Organic Frameworks: Synthesis and Applications
Canadian institutionsUniversity of Calgary
FundersNatural Sciences and Engineering Research Council of CanadaCanada First Research Excellence FundUniversity of Calgary
KeywordsZeolitic imidazolate frameworkMaterials scienceAdsorptionChemical engineeringPolyacrylamideAqueous solutionFourier transform infrared spectroscopyImidazolateX-ray photoelectron spectroscopyComposite numberMetal-organic frameworkOrganic chemistryComposite materialPolymer chemistryChemistry

Abstract

fetched live from OpenAlex

Abstract Metal–organic frameworks (MOFs) have attracted a lot of attention in recent years because of their high surface area and tunable porosities, which allow them to serve as excellent and versatile adsorbents for pollutants in water/wastewater. One of the demanding challenges of using MOFs is that they need to be supported on a substrate or in a matrix to be easier to operate and more efficiently used. This work presents a simple in situ method of synthesizing one of the most popular MOF particles, zeolitic imidazolate framework 8 (ZIF‐8), in a polyacrylamide (PAM) hydrogel using a zinc hydroxide PAM composite as a precursor gel. Characterization of the prepared ZIF‐8 PAM composite hydrogel by scanning electron microscope, energy‐dispersive X‐ray spectroscopy, X‐ray powder diffraction, Fourier‐transform infrared spectroscopy, and X‐ray photoelectron spectroscopy confirms the successful synthesis of ZIF‐8 particles on the surface of and inside the PAM hydrogel. To test the potential of this novel material as an adsorbent, its ability to remove humic acid (HA), a model organic pollutant, from water is evaluated. The maximum adsorption capacity for HA is found to be 111.5 ± 3.0 mg g−1 ZIF‐8, comparable to the performance of other adsorbents for the removal of HA.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.293
Teacher spread0.282 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations81
Published2019
Admission routes2
Has abstractyes

Explore more

Same venueAdvanced Materials InterfacesSame topicMetal-Organic Frameworks: Synthesis and ApplicationsFrench-language works237,207