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Record W2914153404 · doi:10.1002/cjce.23472

Synthesis, characterization, and evaluation of high selectivity mixed molybdenum and vanadium oxide catalysts for oxidative dehydrogenation of propane

2019· article· en· W2914153404 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

venuePublished in a venue whose home country is Canada.
no affNo Canadian affiliation: this work is invisible to an affiliation-only frame.
No Canadian affiliation. An affiliation-only frame, the usual design, would never have seen this work. It is one of the works that make the case for inverting the frame.

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2019
Typearticle
Languageen
FieldChemical Engineering
TopicCatalysis and Oxidation Reactions
Canadian institutionsnot available
Fundersnot available
KeywordsCatalysisDehydrogenationVanadiumMolybdenumSelectivityPropaneInorganic chemistryVanadium oxideChemistryMaterials scienceOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Molybdenum and vanadium oxide catalysts with varied compositions (Mo/V = 1/1, 7/3, 8/2, and 9/1) were prepared using a modified citrate‐nitrate auto‐combustion method for the oxidative dehydrogenation of propane to propylene. These catalysts were characterized by BET‐technique, TPR, XRD, SEM, Raman, and UV spectroscopy. The effects of washing and supercritical CO 2 drying on catalysts during the preparation steps were investigated. Results show an interaction between the molybdenum and vanadium metal ions in all of these catalysts due to the presence of a peak at 785 cm −1 from the Raman study, which was assigned to a polymolybdovanadate species V‐O‐Mo vibration. This interaction could be efficient for alkane activation reaction. The catalysts were evaluated in a fixed bed micro‐reactor at temperatures in the range of 350–600 °C and at atmospheric pressure. The activity of the catalyst increased by increasing the molybdenum content. All of the catalysts in this study showed 100 % selectivity for propylene in the temperature range of 350–450 °C; however, the propylene selectivity was found to decrease with an increase in the temperature. The highest yield of 4.8 % with 100 % propylene selectivity was obtained for a catalyst with Mo/V ratio of 9:1 at 500 °C.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.044
Threshold uncertainty score0.334

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.204
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it