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Study on Thermal Stability of Ceria-Supported Rhodium Catalysts

2019· article· en· W2925820624 on OpenAlexaff
Roman M. Kenzhin, Evgeny A. Alikin, Sergey Denisov, Aleksey A. Vedyagin

Bibliographic record

VenueMaterials science forum · 2019
Typearticle
Languageen
FieldMaterials Science
TopicCatalytic Processes in Materials Science
Canadian institutionsCATAAlliance
Fundersnot available
KeywordsRhodiumCatalysisMaterials scienceThermal stabilityChemical engineeringAqueous solutionAdsorptionInorganic chemistryChemistryOrganic chemistry

Abstract

fetched live from OpenAlex

In the present work, the impact of the rhodium deposition on the thermal stability of ceria-based catalysts was studied. The samples were prepared by an incipient wetness impregnation of the support with aqueous solution of rhodium nitrate. The loading of Rh was 0.1 and 1 wt.%. The textural characteristics of the samples were examined by a low-temperature nitrogen adsorption. It was shown that the addition of rhodium intensifies the process of ceria agglomeration, which leads to the lower values of specific surface area along with increased average pore diameter after the aging at 1000 °C. Stability of the catalysts was investigated by means of a prompt thermal aging procedure. The high-loaded catalyst (1 wt.% Rh/CeO 2 ) was more active than the 0.1 wt.% Rh/CeO 2 sample, while the stability of both the catalysts was excellent. It should be emphasized that the alumina-based reference samples with the similar rhodium loading were significantly less active and poorly stable.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.006
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0060.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.002
Scholarly communication0.0010.001
Open science0.0030.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0050.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.282
Teacher spread0.262 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2019
Admission routes1
Has abstractyes

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