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Record W2944186058 · doi:10.1002/ep.13253

Efficient adsorption of Cd(ІІ) ions from aqueous media onto a semi‐interpenetrating bio‐composite

2019· article· en· W2944186058 on OpenAlexaff
Ahmed M. Shehab, El-Sayed M. Abdel-Bary, Ibrahim M. El‐Sherbiny, Ian S. Butler, Sahar I. Mostafa

Bibliographic record

VenueEnvironmental Progress & Sustainable Energy · 2019
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsMcGill University
Fundersnot available
KeywordsAqueous solutionLangmuir adsorption modelPolyacrylonitrileAdsorptionSorbentNuclear chemistryFourier transform infrared spectroscopyDesorptionChemistryMaterials sciencePolymer chemistryChemical engineeringPhysical chemistryOrganic chemistryPolymer

Abstract

fetched live from OpenAlex

Abstract New bio‐composite, semi‐interpenetrating biopolymers (obtained from hydrolyzed carboxymethyl cellulose grafted polyacrylonitrile [h‐CMC‐g‐PAN] and sodium alginate [Na‐Alg] using CaCl 2 as a cross linker; semi‐interpenetrating biopolymers [s‐IPNs]) have been prepared and fully characterized using spectroscopic (FTIR, scanning electron microscopy, EDS), elemental analysis, and thermal analysis measurements measurements. The morphology and structure of these s‐IPNs are different from those obtained with solely h‐CMC‐g‐PAN and Na‐Alg indicating successive functionalization. The availability of the functional‐rich bio‐composites has afforded an excellent opportunity to test them as sorbents for the uptake of toxic Cd(II) ions from aqueous media. Subsequently, the uptake of Cd(II) ions was shown to be dependent on the pH, shaking time, temperature, amount of sorbent, and the initial concentration of the Cd(II) ions. The maximum Cd(II) ion uptake was 99.5% at pH 6, using 50 mg of sorbent with 120 min shaking time at 25°C. The adsorption isotherm fitted well with Langmuir model, with calculated maximum adsorption capacity 49.75 mg g −1 . The kinetic studies were modeled using a pseudo second‐order reaction. The thermodynamic parameters (Δ H o , Δ G o , and Δ S o ) of the uptake of Cd(II) ions onto s‐IPNs were found to be −13,176.07 Jmol −1 , −4,572.7 Jmol −1 , and 28.87 J K −1 mol −1 , respectively, verifying spontaneous exothermic process. Successive desorption and reusability of s‐IPNs for the uptake of Cd(II) indicated, its high efficiency over three cycles.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.517
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0100.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.188
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations6
Published2019
Admission routes1
Has abstractyes

Explore more

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