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Record W2944544340 · doi:10.1002/app.47936

Crystallization of triethyl‐citrate‐plasticized poly(lactic acid) induced by chitin nanocrystals

2019· article· en· W2944544340 on OpenAlex
Shikha Singh, Ma Lluïsa Maspoch Rulduà, Kristiina Oksman

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueJournal of Applied Polymer Science · 2019
Typearticle
Languageen
FieldMaterials Science
Topicbiodegradable polymer synthesis and properties
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsCrystallizationCrystallinityDifferential scanning calorimetryNucleationMaterials scienceScanning electron microscopeChemical engineeringNanocrystalOptical microscopePolymer chemistryCrystallographyChemistryNanotechnologyComposite materialOrganic chemistry

Abstract

fetched live from OpenAlex

ABSTRACT The aim of this study was to gain a better understanding of the crystallization behavior of triethyl‐citrate‐plasticized poly(lactic acid) (PLA–TEC) in the presence of chitin nanocrystals (ChNCs). The isothermal crystallization behavior of PLA–TEC was studied by polarized optical microscopy, scanning electron microscopy, differential scanning calorimetry, and X‐ray diffraction (XRD). Interestingly, the addition of just 1 wt % ChNCs in PLA–TEC increased the crystallization rate in the temperature range of 135–125 °C. The microscopy studies confirmed the presence of at least three distinct types of spherulites: negative, neutral, and ring banded. The ChNCs also increased the degree of crystallinity up to 32%, even at a fast cooling rate of 25 °C min −1 . The XRD studies further revealed the nucleation effect induced by the addition of ChNCs and thus explained the faster crystallization rate. To conclude, the addition of a small amount (1 wt %) of ChNC to plasticized PLA significantly affected its nucleation, crystal size, and crystallization speed; therefore, the proposed route can be considered suitable for improving the crystallization behavior of PLA. © 2019 Wiley Periodicals, Inc. J. Appl. Polym. Sci. 2019 , 136 , 47936.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score0.834

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.224
Teacher spread0.211 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it