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Record W2945066796 · doi:10.1021/acs.jchemed.8b00618

Room-Temperature Synthesis of Size-Uniform Polystyrene Latex and Characterization of Its Properties: Third-Year Undergraduate Teaching Lab

2019· article· en· W2945066796 on OpenAlexafffund
Nimer Murshid, Nicole Cathcart, Vladimir Kitaev

Bibliographic record

VenueJournal of Chemical Education · 2019
Typearticle
Languageen
FieldChemistry
TopicVarious Chemistry Research Topics
Canadian institutionsWilfrid Laurier University
FundersUniversity of TorontoGovernment of OntarioNatural Sciences and Engineering Research Council of CanadaWilfrid Laurier University
KeywordsEmulsion polymerizationDispersityMaterials sciencePolystyreneChemical engineeringPolymerizationParticle sizePolymerCharacterization (materials science)Polymer chemistryNanotechnologyComposite material

Abstract

fetched live from OpenAlex

Teaching emulsion polymerization is an important benchmark in undergraduate polymer courses. However, the introduction of hands-on experiments in undergraduate polymer laboratories is challenging: experimental time, reagents, and equipment involved are the primary restraints. We report a practical emulsion polymerization laboratory experiment for undergraduate students that includes the synthesis of polystyrene (PS) latex and exposure to multiple methods of characterization. Using a room-temperature redox initiation system of ascorbic acid (vitamin C) and hydrogen peroxide, and scaling the reaction down to ca. 10 mL, simplifies stirring and degassing and alleviates the aforementioned challenges. To prepare latex samples with different sizes and low size dispersity, students explore an effect of a steric stabilizer (polyvinylpyrrolidone, PVP). For effective time management, students perform characterization of previously prepared latex, while qualitatively and quantitatively monitoring particle growth during polymerization stages. Latex characterization performed by students includes measurements of average particle size and zeta potential, estimating conversion and preparation of latex films with determination of glass transition temperature ( T g ). Other characterization methods that can be incorporated in the extended experiments include electron microscopy, atomic force microscopy, and other techniques of colloidal and polymer characterization. Additionally, the prepared latex is able to form colloidal photonic crystal films, enabling size evaluation by color or UV–vis measurements, where selective reflection of blue, green, and red corresponds to latex with particle diameters of 185, 240, and 300 nm, respectively. On the basis of the lab evaluation survey, students performing the experiment have an overall positive learning experience with 94% satisfaction rate.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.007
Threshold uncertainty score0.022

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0070.004

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.244
Teacher spread0.236 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations10
Published2019
Admission routes2
Has abstractyes

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