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Record W2949867930 · doi:10.1021/cm0503073

Melilite-Type Borates Bi<sub>2</sub>ZnB<sub>2</sub>O<sub>7</sub> and CaBiGaB<sub>2</sub>O<sub>7</sub>

2005· article· pt· W2949867930 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueChemistry of Materials · 2005
Typearticle
Languagept
FieldMaterials Science
TopicCrystal Structures and Properties
Canadian institutionsMcMaster UniversityNational Research Council Canada
Fundersnot available
KeywordsOrthorhombic crystal systemCrystallographyBoronMeliliteTetragonal crystal systemSpace groupRietveld refinementCrystal structureNeutron diffractionMaterials sciencePowder diffractionBismuthSuperstructureX-ray crystallographyChemistryDiffractionPhysics

Abstract

fetched live from OpenAlex

The bismuth borates Bi 2 ZnB 2 O 7 and CaBiGaB 2 O 7 have been synthesized by solid-state reactions at temperatures in the 650−825 °C range at 1 atm pressure. These compounds are the only synthetic diborate members of the melilite family, A 2 XZ 2 O 7, in which layers of A cations alternate with XZ 2 O 7 tetrahedral layers. Except for CdBiGaB 2 O 7, the synthesis of other substituted bismuth borate melilites has been unsuccessful. The crystal structures of Bi 2 ZnB 2 O 7 and CaBiGaB 2 O 7 have been determined by powder X-ray diffraction and refined by the Rietveld method using powder neutron diffraction data. CaBiGaB 2 O 7 adopts the regular tetragonal melilite structure ( P 4̄2 1 m space group, Z = 2) containing B 2 O 7 tetrahedral dimers. The refinement of split eight-coordinated sites for the Ca 2+ and Bi 3+ interlayer cations suggests the presence of additional disorder. Bi 2 ZnB 2 O 7 adopts a unique orthorhombic melilite superstructure ( Pba 2 space group, Z = 4) containing both tetrahedral B 2 O 7 and triangular B 2 O 5 dimers. The Bi 3+ cations occupy two distinct interlayer sites with strongly asymmetric 6-fold coordination environments. The preliminary measurement of second harmonic generation efficiencies ( d eff ) of powder samples has yielded values of 4.0 (Bi 2 ZnB 2 O 7 ) and 1.6 (CaBiGaB 2 O 7 ) relative to a KH 2 PO 4 standard.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.004
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Science and technology studies, Scholarly communication, Research integrity, Insufficient payload (model declined to judge)
Consensus categoriesMeta-epidemiology (narrow), Science and technology studies
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.014
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0040.002
Meta-epidemiology (narrow)0.0040.004
Meta-epidemiology (broad)0.0050.001
Bibliometrics0.0010.002
Science and technology studies0.0020.003
Scholarly communication0.0030.002
Open science0.0030.003
Research integrity0.0030.001
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.223
Teacher spread0.210 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it