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Record W2951261205 · doi:10.3390/catal9060542

Catalyst/Feedstock Ratio Effect on FCC Using Different Catalysts Samples

2019· article· en· W2951261205 on OpenAlexafffund
Abdualkaber Alkhlel, Hugo de Lasa

Bibliographic record

VenueCatalysts · 2019
Typearticle
Languageen
FieldChemistry
TopicZeolite Catalysis and Synthesis
Canadian institutionsWestern University
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCatalysisFluid catalytic crackingCokeCrackingBenzeneMaterials scienceChemical engineeringChemistryMetallurgyOrganic chemistry

Abstract

fetched live from OpenAlex

The present study is a follow-up to a recent authors contribution which describes the effect of the C/O (catalyst/oil) ratio on catalytic cracking activity and catalyst deactivation. This study, while valuable, was limited to one fluidized catalytic cracking (FCC) catalyst. The aim of the present study is to consider the C/O effect using three FCC catalysts with different activities and acidities. Catalysts were characterized in terms of crystallinity, total acidity, specific surface Area (SSA), temperature programmed ammonia desorption (NH3-TPD), and pyridine chemisorption. 1,3,5-TIPB (1,3,5-tri-isopropyl benzene) catalytic cracking runs were carried out in a bench-scale mini-fluidized batch unit CREC (chemical reactor engineering centre) riser simulator. All data were taken at 550 °C with a contact time of 7 s. Every experiment involved 0.2 g of 1,3,5-TIPB with the amount of catalyst changing in the 0.12–1 g range. The resulting 0.6–5 g oil/g cat ratios showed a consistent 1,3,5-TIPB conversion increasing first, then stabilizing, and finally decreasing modestly. On the other hand, coke formation and undesirable benzene selectivity always rose. Thus, the reported results show that catalyst density affects both catalyst coking and deactivation, displaying an optimum C/O ratio, achieving maximum hydrocarbon conversions in FCC units.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.018
GPT teacher head0.245
Teacher spread0.227 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations9
Published2019
Admission routes2
Has abstractyes

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