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Record W2951290680 · doi:10.48550/arxiv.1206.2617

Defect Textures in Polygonal Arrangements of Cylindrical Inclusions in Cholesteric Liquid Crystal Matrices

2012· preprint· en· W2951290680 on OpenAlexaff
Yogesh K. Murugesan, Damiano Pasini, Alejandro D. Rey

Bibliographic record

VenuearXiv (Cornell University) · 2012
Typepreprint
Languageen
FieldMaterials Science
TopicLiquid Crystal Research Advancements
Canadian institutionsMcGill University
FundersBasic Energy SciencesU.S. Department of Energy
KeywordsMaterials scienceLiquid crystalChirality (physics)Elastic energyTopological defectPhase (matter)Condensed matter physicsTexture (cosmology)CrystallographyParticle (ecology)AnisotropyPhase transitionMatrix (chemical analysis)Chemical physicsOpticsComposite materialPhysicsSymmetry breakingChemistryChiral symmetry breakingThermodynamics

Abstract

fetched live from OpenAlex

A systematic computational and scaling analysis of defect textures in polygonal arrangement of cylindrical particles embedded in a cholesteric (Ch) liquid crystal matrix is performed using the Landau de Gennes model for chiral self assembly, with strong anchoring at the particles' surface. The defect textures and LC phases observed are investigated as a function of chirality, elastic anisotropy, particle polygonal arrangement and particle size. The presence of a polygonal network made of N circular inclusions results in defect textures of a net charge of -(N-2)/2 per unit polygonal cell. As the chirality increases, the LC matrix shows the following transition sequence: weakly twisted cholesterics, 2D blue phases with non-singular/ singular defect lattices, cholesteric phases with only disclinations, and fingerprint cholesteric textures with disclinations and dislocations. For monomeric mesogens at concentrations far from the I/Ch phase transition and low chirality, for a given symmetry of the LC phase, the particle with weaker (stronger) confinement results in a phase with lower (higher) elastic energy, while at high chirality the elastic energy of a LC phase is proportional to the number of particles that form the polygonal network. Thus, hexagonal (triangular) particle arrangement results in low elastic energy at low (high) chirality. For semiflexible polymeric mesogens (high elastic anisotropy), defect textures with fewer disclinations/ dislocations arise but due to layer distortions we find a higher elastic energy than monomeric mesogens. The defects arising in the simulations and the texture rules established are in agreement with experimental observations in cellulosic liquid crystal analogues such as plant cell wall and helical biological polymeric mesophases made of DNA, PBLG and xanthan.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.565
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0010.001
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0010.004
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.067
GPT teacher head0.250
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2012
Admission routes1
Has abstractyes

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