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Record W2952592291 · doi:10.1021/cm020803g

Synthesis, Structure, and Physical Properties of Mixed Valent Mo<sub>2</sub>SbS<sub>2</sub>, the First Superconducting Antimonide-Sulfide

2003· article· en· W2952592291 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueChemistry of Materials · 2003
Typearticle
Languageen
FieldMaterials Science
TopicIron-based superconductors research
Canadian institutionsBrockhouse Institute for Materials ResearchMcMaster UniversityUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsMonoclinic crystal systemIsostructuralAntimonideCrystallographyMaterials scienceMagnetic susceptibilityCrystal structureSuperconductivitySeebeck coefficientElectronic band structureSulfideBand gapStoichiometryFerrimagnetismChemistryCondensed matter physicsPhysical chemistryMagnetizationMetallurgy

Abstract

fetched live from OpenAlex

We identified a new ternary molybdenum antimonide-sulfide, Mo 2 SbS 2 . Black, needle-shaped crystals of Mo 2 SbS 2 can be synthesized by reacting stoichiometric amounts of the elements at 850 °C for 7 days with I 2 (<2 wt %) as the transporting reagent; however, the crystals of Mo 2 SbS 2 are too small for a single-crystal structure investigation. Therefore, the crystal structure of Mo 2 SbS 2 was analyzed by powder X-ray diffraction using Rietveld refinements. The compound crystallizes in a monoclinic system (space group P 2 1 / m, a = 6.50920(7) Å, b = 3.18231(4) Å, c = 9.3548(1) Å, β = 105.4430(8)°, Z = 2). The title compound is isostructural with Mo 2 S 3; and the Mo−Mo, Mo−Sb, and Mo−S distances are comparable with those in MoSb 2 S. The results from the Seebeck coefficient and magnetic susceptibility measurements and electronic band structure calculations suggest metallic behavior. The band structure of Mo 2 SbS 2 exhibits van Hove singularities hinting at superconductivity, which was subsequently confirmed via magnetic susceptibility measurements.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.002
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.002
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.023
GPT teacher head0.232
Teacher spread0.209 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it