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Record W2969619070 · doi:10.1002/0471264229.os096.18

Three‐Step Synthesis of 2‐(Diiodomethyl)‐4,4,5,5‐Tetramethyl‐1,3,2‐Dioxaborolane from Dichloromethane

2020· other· en· W2969619070 on OpenAlexaff
Morgane Sayes, Guillaume Benoît, André B. Charette

Bibliographic record

VenueOrganic Syntheses · 2020
Typeother
Languageen
FieldChemistry
TopicOrganoboron and organosilicon chemistry
Canadian institutionsUniversité de MontréalCentre in Green Chemistry and Catalysis
Fundersnot available
KeywordsDichloromethaneCyclopropaneChemistryReagentRing (chemistry)ChromiumCombinatorial chemistryOrganic chemistryFunctional groupSolvent

Abstract

fetched live from OpenAlex

Abstract 2‐(diiodomethyl)‐4,4,5,5‐tetramethyl‐1,3,2‐dioxaborolane is used to perform direct borocyclopropanation reactions; direct meaning that the cyclopropane ring is formed at the same time as the boronic ester is installed. This article describes the procedure for the synthesis of 2‐(diiodomethyl)‐4,4,5,5‐tetramethyl‐1,3,2‐dioxaborolane from dichloromethane. It presents some of the important points to be considered, the conditions that need to be maintained, characterization data, and the reagents required, as well as the techniques used and the equipment setup that are vital to carrying out the process. 2‐(diiodomethyl)‐4,4,5,5‐tetramethyl‐1,3,2‐dioxaborolane has been used in a chromium‐promoted borocyclopropanation. This methodology is applicable to unactivated alkenes under mild conditions with good stereoselectivities and good functional group tolerance. The article also describes the hazards associated with working with chemicals and the ways to deal with these hazards.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.004
Threshold uncertainty score0.013

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0040.002

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.222
Teacher spread0.208 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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