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Record W2971730989 · doi:10.1002/macp.201900234

Soluble Telechelic Polycondensation Poly(ether ketones): Synthesis and Characterization

2019· article· en· W2971730989 on OpenAlex
Abdelkader Benhalima, Alexandra Fürtös, Josée Brisson

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueMacromolecular Chemistry and Physics · 2019
Typearticle
Languageen
FieldMaterials Science
TopicSynthesis and properties of polymers
Canadian institutionsUniversité de MontréalUniversité Laval
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsCondensation polymerPolymer chemistryEtherChemistryDifferential scanning calorimetryGel permeation chromatographyThermogravimetryCrystallizationPolymerReactivity (psychology)SolventOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract The present article reports the synthesis of soluble, propyl‐substituted aromatic ring telechelic polycondensation blocks having molecular weights ranging from 1800 to 6500 g mol −1 and polymolecularities of 1.3 to 1.7. Chain‐growth polycondensation is performed, and the initiator is selected through reactivity studies, using 19 F nuclear magnetic resonance (NMR) measurements. Gel permeation chromatography, NMR spectroscopy, and matrix‐assisted laser desorption/ionization time of flight mass spectrometry show that blocks are terminated by a methoxy group at one end and a fluorine atom at the other. Polymers are crystalline as synthesized, as shown by X‐ray diffraction and differential scanning calorimetry, do not recrystallize once melted, and undergo solvent‐induced crystallization. Crystalline peak positions and relative intensities are different from those observed for other poly(ether ketones). The difference in crystal form is proposed to stem from packing disruption related to the presence of propyl substituents. Thermogravimetry shows a good thermal resistance up to 450 °C.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.019
Threshold uncertainty score0.673

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.194
Teacher spread0.187 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it