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Record W2973230909 · doi:10.1002/0471264229.os096.22

Stereoselective Synthesis of ( <i>R</i> )‐(( <i>R</i> )‐1‐Phenyl‐2,2,2‐Trichloroethyl)2‐(2‐Bromophenyl)aziridine‐1‐Carboxylate

2020· other· en· W2973230909 on OpenAlexaff
H. Lebel, Henri Piras

Bibliographic record

VenueOrganic Syntheses · 2020
Typeother
Languageen
FieldChemistry
TopicSynthesis and Catalytic Reactions
Canadian institutionsUniversité de Montréal
Fundersnot available
KeywordsAziridineChemistryMoietyCarbamateStereoselectivityCleavage (geology)CarboxylateCombinatorial chemistryReagentAnilineNitreneOrganic chemistryMedicinal chemistryRing (chemistry)Catalysis

Abstract

fetched live from OpenAlex

Abstract This chapter article the procedure for synthesis of (R)‐((R)‐1‐phenyl‐2,2,2‐trichloroethyl)2‐(2‐bromophenyl)aziridine‐1‐carboxylate. It presents some of the important points to be considered, the conditions that need to be maintained, characterization data, and the reagents required, as well as the techniques used and the equipment setup that are vital to carrying out the process. Stereoselective aminations of alkenes and alkanes are achieved using namely metal nitrene species. The scope of the aziridination reaction includes styrene derivatives containing diversely functionalized aromatic ring as well as β‐methylstyrene. The cleavage of the (R)‐2,2,2‐trichloro‐1‐phenylethyl carbamate undergoes under basic reaction conditions, avoiding the concomitant opening of the aziridine moiety, that is typically observed for cleavage of sulfonyl‐protected aziridines. The article also describes the hazards associated with working with chemicals and the ways to deal with these hazards.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.003
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesInsufficient payload (model declined to judge)
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Not applicable · Consensus signal: none
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.462
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.003
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0660.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.215
Teacher spread0.202 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; both teacher heads agree on what is shown here.

Study designNot applicable
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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