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Record W2973437029 · doi:10.1002/admi.201901456

Reaction and Energy Levels at Oxide–Oxide Heterojunction Interfaces

2019· article· en· W2973437029 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueAdvanced Materials Interfaces · 2019
Typearticle
Languageen
FieldMaterials Science
TopicElectronic and Structural Properties of Oxides
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsHeterojunctionOxideMaterials scienceBand bendingDipoleRedoxWork functionCatalysisWork (physics)Interface (matter)NanotechnologyChemical physicsOptoelectronicsChemical engineeringChemistryLayer (electronics)Composite material

Abstract

fetched live from OpenAlex

Abstract Oxide–oxide heterojunction interfaces (OHIs) are foundations for many applications such as transistors, optoelectronic devices, and chemical catalysis. The formation of OHIs involves complex events such as charge transfer, interfacial diffusion, and chemical reactions. These events collectively contribute to an OHI's energy structure and to its ability to perform an intended application. Here, multiple MoO 3 /oxide interfaces are studied at which changes in multiple oxidation states Mo x + can be easily tracked. For the formation of reactive interfaces, it is found that the primary driving force behind the reduction of MoO 3 is redox reactions at the interfaces. For the nonreactive interface, the reduction of MoO 3 occurs as a result of various factors such as oxygen deficiency. At these OHIs, band bending and formation of interface dipole are observed. It is discovered that the degrees of interface dipole and work function at the OHIs scale linearly as a function of the contacting oxide's work function. These findings provide the guide in designing OHIs for a specific application.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.231
Teacher spread0.219 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it