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Hygroscopic Properties of Calcium Chloride and Its Role on Cold-End Corrosion in Biomass Combustion

2019· article· en· W2977199138 on OpenAlexaff
Emil Vainio, Nikolai DeMartini, Leena Hupa, Lars-Erik Åmand, Tobias Richards, Mikko Hupa

Bibliographic record

VenueEnergy & Fuels · 2019
Typearticle
Languageen
FieldEngineering
TopicMetallurgical Processes and Thermodynamics
Canadian institutionsUniversity of Toronto
FundersAcademy of Finland
KeywordsCorrosionChemistryFlue gasChlorideRelative humidityInorganic chemistryWater vaporChemical engineeringMaterials scienceMetallurgy

Abstract

fetched live from OpenAlex

In biomass combustion, hygroscopic and deliquescent salts may cause cold-end corrosion and operational problems, such as deposit buildup and decrease in heat transfer. Calcium chloride is a deliquescent salt that can be found in the cold-end of boilers. In this study, the hygroscopic properties and corrosiveness of CaCl 2 in flue gas conditions were studied. The formation of hydrates and the deliquescent properties of CaCl 2 were studied with various techniques. The hydrate formation, deliquescence, and water absorption at various temperatures, humidities, and cooling rates were studied using thermogravimetric analysis. A stable flow of water vapor (5–35 vol %) was created with a membrane humidifier with a humidity sensor. Deliquescence and recrystallization of CaCl 2 were determined by a two-electrode chronoamperometric setup. The effect of mixtures containing CaCl 2, CaCO 3, and CaSO 4 on deliquescence was also studied. Furthermore, the corrosivity of CaCl 2 on mild steel was studied above and below the deliquescence temperature, and the corrosion products were analyzed by means of scanning electron microscopy with energy dispersive X-ray spectroscopy (SEM-EDX). This work revealed that both deliquescence and recrystallization of CaCl 2 are of importance when assessing the corrosivity of the salt. When deliquescence occurred, the corrosion rate was substantial, and the corrosion rate was dependent on the ion concentration of the formed solution. Drying or crystallization of the salt solution occurred at 35–42 °C higher than the deliquescence temperature with 10–35 vol % H 2 O. Thus, large variations in the flue gas water vapor concentration will impact the wetting and drying of the salt. The observations presented in this paper give guidelines on how to prevent corrosion caused by deliquescent CaCl 2 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.009

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.011
GPT teacher head0.195
Teacher spread0.184 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations37
Published2019
Admission routes1
Has abstractyes

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