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Record W2977921622 · doi:10.6000/1929-5030.2019.08.02

How to Resolve the Problem of Drago's Four Parameters in the Context of Molecular Interactions

2019· article· en· W2977921622 on OpenAlexvenueno aff
Ho Nam Tran, Michel Buchmann

Bibliographic record

VenueJournal of Applied Solution Chemistry and Modeling · 2019
Typearticle
Languageen
FieldChemistry
TopicChemical Thermodynamics and Molecular Structure
Canadian institutionsnot available
Fundersnot available
KeywordsContext (archaeology)PsychologyGeographyArchaeology

Abstract

fetched live from OpenAlex

This study aims to provide a new thermodynamic method for determining the value of Drago's four interaction parameters, namely Ea, Eb, Ca, and Cb (kcal1/2 mol-1/2). The method is based on the following fundamental novelties: The values of the parameters Ea, Eb, Ca, and Cb are simultaneously determined for seven amphoteric substances. Thus, there are a total of 28 values to be determined, with each set consisting of seven substances. For the seven selected amphoteric substances, there are seven equations of the type: V∂2h / n = (Ea Eb + Ca Cb) Next, all possible 2-to-2 combinations of these seven substances are generated. For each 2-to-2 combination, one of the two is selected as a solute (2) and the other as a solvent (1), or vice versa. By measuring the mixing energy, ΔEmix (2.1), of these combinations, the 21 measurements available to extract the energy, ΔEint, of chemical bonds, according to the enclosed Buchmann paper: ΔEmix (2.1) = (Ea1 Eb2 + Ca1 Cb2) + (Ea2 Eb1 + Ca2 Cb1) Next, the seven equalities of the type V∂2h / nj = (Eaj Ebj + Caj Cbj) (kJ / mol) with j = 1,7 are put together with 21 equalities of the type ΔEint = (Eaj Ebj+1 + Caj Cbj+1) + (Eaj+1 Ebj + Caj+1 Cbj). This will generate a system comprising 28 equations for 28 unknown parameters. The resolution of this system will afford the 28 sought values of Drago's four parameters Ea, Eb, Ca, Cb for the seven selected substances.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.028
Threshold uncertainty score0.283

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.234
Teacher spread0.220 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2019
Admission routes1
Has abstractyes

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