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Record W2980430176 · doi:10.1021/acssensors.9b01307

On MoS<sub>2</sub> Thin-Film Transistor Design Consideration for a NO<sub>2</sub> Gas Sensor

2019· article· en· W2980430176 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueACS Sensors · 2019
Typearticle
Languageen
FieldEngineering
TopicNanowire Synthesis and Applications
Canadian institutionsUniversity of Waterloo
FundersNatural Sciences and Engineering Research Council of CanadaNational Research Foundation of Korea
KeywordsPassivationMaterials scienceThin-film transistorOptoelectronicsThreshold voltageTransistorSchottky barrierVoltageLayer (electronics)NanotechnologyElectrical engineering

Abstract

fetched live from OpenAlex

MoS2 thin-film transistors (TFTs) are fabricated and simulated to explore the NO2 gas sensing mechanism depending on different device structures. In particular, the role of the Al2O3 passivation layer on the MoS2 channel has been investigated. In the case of nonpassivated MoS2 TFTs, increase of off-current is observed with NO2 gas, which has been modeled with the modulation of the effective Schottky barrier height for holes because of the generation of in-gap states near the valence band as NO2 gases interact with the MoS2 channel. The nonpassivated MoS2 TFTs are simulated based on nonequilibrium Green’s function method, and the simulation results do confirm this sensing mechanism. On the other hand, MoS2 TFTs with the Al2O3 passivation layer have been modeled with a pseudo-double gate structure as NO2 gases on the capping layer can act like the secondary gate inducing the positive charge state. Our quantum transport simulation shows that the significant threshold voltage shift can be achieved with NO2 gas, which matches the experimental observation, thereby exhibiting a completely different sensing mechanism of the passivated device from the nonpassivated counterpart. In addition, we also discuss competing device parameters for the passivated MoS2 TFTs by varying the main and the secondary gate dielectric, suggesting co-optimization to realize high sensitivity and low power consumption simultaneously.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.034
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.012
GPT teacher head0.202
Teacher spread0.190 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it