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Record W2989265416 · doi:10.1139/cjp-2019-0475

The smell of coffee: the carbon atom microwave structure of coffee furanone validated by quantum chemistry

2019· article· en· W2989265416 on OpenAlexvenueno aff
Vinh Van, Wolfgang Stahl, Minh Tuyen Nguyen, Ha Vinh Lam Nguyen

Bibliographic record

VenueCanadian Journal of Physics · 2019
Typearticle
Languageen
FieldChemistry
TopicMolecular Spectroscopy and Structure
Canadian institutionsnot available
FundersRWTH Aachen UniversityAgence Nationale de la Recherche
KeywordsIsotopologueConformational isomerismChemistryQuantum chemistrySpectral lineAtom (system on chip)Carbon fibersMicrowaveComputational chemistryRotational spectroscopyFourier transformAnalytical Chemistry (journal)CrystallographyMoleculePhysicsCrystal structureOrganic chemistryMaterials scienceQuantum mechanics

Abstract

fetched live from OpenAlex

The rotational spectra of coffee furanone (2-methyltetrahydrofuran-3-one) have been measured in the frequency range from 2.0 to 26.5 GHz using a molecular jet Fourier transform microwave spectrometer. Quantum chemical calculations used for the conformational analysis yielded two stable twist conformers, which were described using the Cremer–Pople notation for five-membered rings. The experimental spectrum of the more stable conformer with the methyl group in equatorial position was assigned and fitted using a rigid rotor model with centrifugal distortion corrections. The spectra of all five 13 C-isotopologues could be observed in natural abundance. The carbon atom structure was experimentally deduced using Kraitchman’s equations and compared with the structure calculated by quantum chemistry.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.547

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.184
Teacher spread0.182 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2019
Admission routes1
Has abstractyes

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