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Record W2993352709 · doi:10.1002/chem.201904085

Hierarchical Hollow‐Nanocube Ni−Co Skeleton@MoO<sub>3</sub>/MoS<sub>2</sub> Hybrids for Improved‐Performance Lithium‐Ion Batteries

2019· article· en· W2993352709 on OpenAlexaff
Juan Li, Shuang Hou, Tiezhong Liu, Liangke Wang, Mei Chen, Yayun Guo, Lingzhi Zhao

Bibliographic record

VenueChemistry - A European Journal · 2019
Typearticle
Languageen
FieldEngineering
TopicAdvancements in Battery Materials
Canadian institutionsInstitute of Aging
FundersScience and Technology Planning Project of Guangdong Province
KeywordsMaterials scienceAnodeLithium (medication)Raman spectroscopyChemical engineeringPrussian bluePrecipitationParticle sizeHydrothermal circulationMetalNickelPhase (matter)AlloyElectrochemistryNanotechnologyMetallurgyElectrodeChemistry

Abstract

fetched live from OpenAlex

Abstract Improving the performance of anode materials for lithium‐ion batteries (LIBs) is a hotly debated topic. Herein, hollow Ni−Co skeleton@MoS2/MoO3 nanocubes (NCM‐NCs), with an average size of about 193 nm, have been synthesized through a facile hydrothermal reaction. Specifically, MoO3/MoS2 composites are grown on Ni−Co skeletons derived from nickel–cobalt Prussian blue analogue nanocubes (Ni−Co PBAs). The Ni−Co PBAs were synthesized through a precipitation method and utilized as self‐templates that provided a larger specific surface area for the adhesion of MoO3/MoS2 composites. According to Raman spectroscopy results, as‐obtained defect‐rich MoS2 is confirmed to be a metallic 1T‐phase MoS2. Furthermore, the average particle size of Ni−Co PBAs (≈43 nm) is only about one‐tenth of the previously reported particle size (≈400 nm). If assessed as anodes of LIBs, the hollow NCM‐NC hybrids deliver an excellent rate performance and superior cycling performance (with an initial discharge capacity of 1526.3 mAh g−1 and up to 1720.6 mAh g−1 after 317 cycles under a current density of 0.2 A g−1). Meanwhile, ultralong cycling life is retained, even at high current densities (776.6 mAh g−1 at 2 A g−1 after 700 cycles and 584.8 mAh g−1 at 5 A g−1 after 800 cycles). Moreover, at a rate of 1 A g−1, the average specific capacity is maintained at 661 mAh g−1. Thus, the hierarchical hollow NCM‐NC hybrids with excellent electrochemical performance are a promising anode material for LIBs.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.208
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations20
Published2019
Admission routes1
Has abstractyes

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Same venueChemistry - A European JournalSame topicAdvancements in Battery MaterialsFrench-language works237,207