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Record W2998568404 · doi:10.1103/physrevb.100.245433

Third harmonic generation of undoped graphene in Hartree-Fock approximation

2019· article· en· W2998568404 on OpenAlexafffund
Jinluo Cheng, J. E. Sipe, Chunlei Guo

Bibliographic record

VenuePhysical review. B./Physical review. B · 2019
Typearticle
Languageen
FieldMaterials Science
TopicGraphene research and applications
Canadian institutionsUniversity of Toronto
FundersK. C. Wong Education FoundationChinese Academy of SciencesNatural Sciences and Engineering Research Council of CanadaNational Natural Science Foundation of China
KeywordsGrapheneHartree–Fock methodPhysicsQuantum mechanicsQuantum electrodynamicsCondensed matter physics

Abstract

fetched live from OpenAlex

We theoretically investigate the effects of Coulomb interaction, at the level of the unscreened Hartree-Fock approximation in an equation of motion framework, on third harmonic generation from undoped graphene. The unperturbed electronic states are described by a widely used two-band tight-binding model and the Coulomb interaction is described by the Ohno potential. The ground state is renormalized by taking into account the Hartree-Fock term and the optical conductivities are obtained by numerically solving the equations of motion. The absolute values of conductivity for third-harmonic generation depend on the photon frequency $\mathrm{\ensuremath{\Omega}}$ as ${\mathrm{\ensuremath{\Omega}}}^{\ensuremath{-}n}$ for $\ensuremath{\hbar}\mathrm{\ensuremath{\Omega}}<1$, and then show a peak as $3\ensuremath{\hbar}\mathrm{\ensuremath{\Omega}}$ approaches the renormalized energy of the $M$ point. Taking into account the Coulomb interaction, $n$ is found to be 5.5, which is significantly greater than the value of 4 found with the neglect of the Coulomb interaction. Therefore, the Coulomb interaction enhances third-harmonic generation at low photon energies---for our parameters $\ensuremath{\hbar}\mathrm{\ensuremath{\Omega}}<0.8$ eV---and then reduces it until the photon energy reaches about 2.1 eV. The effect of the background dielectric constant is also considered.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: Simulation or modeling
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.003
Threshold uncertainty score0.007

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.001
Bibliometrics0.0010.000
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0020.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.041
GPT teacher head0.379
Teacher spread0.338 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2019
Admission routes2
Has abstractyes

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Same venuePhysical review. B./Physical review. BSame topicGraphene research and applicationsFrench-language works237,207