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Record W2998633063 · doi:10.1021/acs.jpclett.9b03632

Superconducting Zirconium Polyhydrides at Moderate Pressures

2020· article· en· W2998633063 on OpenAlexafffund
Hui Xie, Wenting Zhang, Defang Duan, Xiaoli Huang, Yanping Huang, Hao Song, Xiaolei Feng, Yansun Yao, Chris J. Pickard, Tian Cui

Bibliographic record

VenueThe Journal of Physical Chemistry Letters · 2020
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicHigh-pressure geophysics and materials
Canadian institutionsUniversity of Saskatchewan
FundersEngineering and Physical Sciences Research CouncilNatural Sciences and Engineering Research Council of CanadaState Administration of Foreign Experts AffairsMinistry of Science and Technology of the People's Republic of ChinaMinistry of Education of the People's Republic of ChinaNational Natural Science Foundation of ChinaRoyal Society
KeywordsIsostructuralSuperconductivityDiamond anvil cellZirconiumMaterials scienceHigh pressureCrystal structureCondensed matter physicsDiffractionSynchrotronCrystallographyChemistryMetallurgyEngineering physicsPhysicsNuclear physics

Abstract

fetched live from OpenAlex

Highly compressed hydrides have been at the forefront of the search for high- T c superconductivity. The recent discovery of record-high T c ’s in H 3 S and LaH 10± x under high pressure fuels the enthusiasm for finding good superconductors in similar hydride groups. Guided by first-principles structure prediction, we successfully synthesized ZrH 3 and Zr 4 H 15 at modest pressures (30–50 GPa) in diamond anvil cells by two different reaction routes: ZrH 2 + H 2 at room temperature and Zr + H 2 at ∼1500 K by laser heating. From the synchrotron X-ray diffraction patterns, ZrH 3 is found to have a Pm 3̅ n structure corresponding to the familiar A15 structure, and Zr 4 H 15 has an I 4̅3 d structure isostructural to Th 4 H 15 . Electrical resistance measurement and the dependence of T c on the applied magnetic field of the sample showed the emergence of two superconducting transitions at 6.4 and 4.0 K at 40 GPa, which correspond to the two T c ’s for ZrH 3 and Zr 4 H 15 .

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.005

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.016
GPT teacher head0.200
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations42
Published2020
Admission routes2
Has abstractyes

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