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Record W3003478964 · doi:10.3389/fbioe.2020.00011

Use of Ionic Liquids in Chitin Biorefinery: A Systematic Review

2020· review· en· W3003478964 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueFrontiers in Bioengineering and Biotechnology · 2020
Typereview
Languageen
FieldEngineering
TopicCatalysis for Biomass Conversion
Canadian institutionsUniversity of Calgary
Fundersnot available
KeywordsBiorefineryIonic liquidChitinBiomass (ecology)Lignocellulosic biomassCelluloseBiopolymerDissolutionChemistryPulp and paper industryBiochemical engineeringOrganic chemistryChemical engineeringPolymerCatalysisRaw materialChitosanEngineeringAgronomy

Abstract

fetched live from OpenAlex

Lignocellulosic biomass biorefinery is the most extensively investigated biorefinery model. At the same time, chitin, structurally similar to cellulose and the second most abundant polymer on Earth, represents a unique chemical structure that allows the direct manufacture of nitrogen-containing building blocks and intermediates, a goal not accomplishable using lignocellulosic biomass. However, the recovery, dissolution, and treatment of chitin was fairly challenging until the polymer's easy dissolution in ionic liquids (salts that are liquid at room temperature) was discovered. In this systematic review, we highlight recent developments in the processing of chitin, with a particular emphasis placed on methods conducted with the help of ionic liquids used as solvents, co-solvents, or catalysts. Such use of ionic liquids in the field of chemical transformations of chitin not only allows for shorter times and less harsh reaction conditions, but also results in different outcomes and higher product yields when compared with reactions conducted in "traditional" manner. Valorization of biomass in general, and chitin in particular, is a key enabling strategy of the circular economy, due to the importance of the sustainable production of biomass-based goods and chemicals and full chain resource efficiency. Economics is driven by the production of high-value chemicals or chemical intermediates from various biomasses, and chitinous biomass is a valuable potential resource. A fundamental "paradigm shift" will radically change the balance of oil-based chemicals to biopolymer-based chemicals, and chitin valorization is a necessary step aimed toward its full market competitiveness and flexibility.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Systematic review · Consensus signal: Systematic review
GenreCandidate signal: Review · Consensus signal: Review
Teacher disagreement score0.325
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0040.000
Bibliometrics0.0020.002
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.015
GPT teacher head0.219
Teacher spread0.204 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it