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Monochloramine Formation and Decay in the Presence of H2O2 after UV/H2O2 Advanced Oxidation

2020· article· en· W3013369097 on OpenAlexaffabout
Chengjin Wang, Liang Zheng, Susan Andrews, Ron Hofmann

Bibliographic record

VenueJournal of Environmental Engineering · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicWater Treatment and Disinfection
Canadian institutionsUniversity of Toronto
Fundersnot available
KeywordsChloramineChlorineChemistryAmmoniaWater treatmentChloraminationHydrogen peroxideEnvironmental chemistryPhotochemistryInorganic chemistryEnvironmental engineeringOrganic chemistryEnvironmental science

Abstract

fetched live from OpenAlex

When treating drinking water using UV/H2O2 advanced oxidation, the H2O2 residual is usually quenched to allow for downstream chlorine stability. In some utilities, monochloramine (NH2Cl) is used for secondary disinfection, and H2O2 may not need to be quenched because NH2Cl and H2O2 can coexist for some time. However, when ammonia and chlorine are applied to form NH2Cl in the H2O2-containing water, H2O2 will compete with ammonia to react with the applied chlorine, compromising the NH2Cl formation efficiency. This research combined theory and experiments to evaluate NH2Cl formation efficiency in the presence of H2O2 in Lake Ontario water and, after NH2Cl formation, its subsequent decay at different temperatures and pH. The results demonstrated that at many typical temperatures and pH, the presence of H2O2 does not significantly impair the formation of NH2Cl. Furthermore, while H2O2 accelerates NH2Cl decay, the results suggest that under specific conditions, such as short to medium residence times (e.g., less than 48 h), it may be possible for NH2Cl to coexist with as much as 5 mg/L H2O2 without compromising secondary disinfection.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.775
Threshold uncertainty score0.213

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.001
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.167
Teacher spread0.163 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations2
Published2020
Admission routes2
Has abstractyes

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