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Structure of the Alternative Complex III from <i>Flavobacterium johnsoniae</i> in a Supercomplex with Cytochrome <i>c</i> Oxidase

2020· article· en· W3016273005 on OpenAlexaffabout
Robert B. Gennis, Chang Sun, Samir Benlekbir, Padmaja Venkatakrishnan, Yuhang Wang, Sangjin Hong, Jonathan P. Hosler, Emad Tajkhorshid, John L. Rubinstein

Bibliographic record

VenueThe FASEB Journal · 2020
Typearticle
Languageen
FieldEnergy
TopicAlgal biology and biofuel production
Canadian institutionsSickKids FoundationHospital for Sick Children
Fundersnot available
KeywordsCoenzyme Q – cytochrome c reductaseProtein subunitChemistryCytochrome c oxidaseElectron Transport Complex IVCytochromeOxidase testCytochrome cCysteineCrystallographyStereochemistryBiochemistryEnzymeMitochondrion

Abstract

fetched live from OpenAlex

Alternative Complex III (ACIII), like Complex III, catalyzes the oxidation of membrane‐bound quinol and reduction of cytochrome c , but is structurally unrelated to Complex III. We solubilized the ACIII directly from membranes of Flavobacterium johnsoniae using styrene maleic acid (SMA) copolymer in the absence of traditional detergents. The ACIII was isolated as a functional 1:1 supercomplex with an aa 3 ‐type cytochrome c oxidase (cyt aa 3 ) within SMA copolymer nanodiscs. We determined the structure of the ACIII component of the supercomplex to 3.4 Å resolution by cryo‐EM and constructed an atomic model for its six subunits, two of which are anchored to the lipid bilayer with N‐terminal triacylated cysteine residues, resolved here for the first time. The structure also contains a [3Fe‐4S] cluster, a [4Fe‐4S] cluster, and six hemes c along with 11 phospholipid molecules. The ACIII is in direct contact with subunit III of the cyt aa 3 component of the supercomplex. The structure revealed that this subunit is structurally modified from the canonical form of subunit III to facilitate association with ACIII, suggesting a specific role of the supercomplex in the respiratory system of this bacterium. Support or Funding Information This work was supported by funds from the National Institutes of Health (R01‐HL16101 to R.B.G., P41‐GM104601, U54‐GM087519, and R01‐GM123455 to E.T.) and Canadian Institutes of Health Research (MOP‐81294 to J.L.R.); J.L.R. was supported by the Canada Research Chairs program. Some of this work was performed at the Simons Electron Microscopy Center and National Resource for Automated Molecular Microscopy, supported by grants from the Simons Foundation (349247), and the National Institute of General Medical Sciences (GM103310, OD019994). Molecular dynamics simulations were performed at Blue Waters (ACI‐1713784 to E.T.) and XSEDE (MCA06N060 to E.T.). Blue Waters is supported by the National Science Foundation (OCI‐0725070 and ACI‐1238993) and the state of Illinois. XSEDE is supported by the National Science Foundation (ACI‐1548562). We thank Mark Mcbride for kindly providing us with the Flavobacterium johnsoniae UW101 strain. We thank Bridget Carragher and Clint Potter for facilitating access to the Titan Krios and Zhening Zhang for collecting data. We also thank Mohammad Mazhab‐Jafari for advice on building atomic models.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score0.012

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0010.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.218
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

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Citations4
Published2020
Admission routes2
Has abstractyes

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