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Record W3033367533 · doi:10.1002/9780470027318.a9689

Inductively Coupled Plasma Mass Spectrometry Analysis of Environmental Samples for the Quantification of Potentially Toxic Species

2020· other· en· W3033367533 on OpenAlexaff
Robert Teuma‐Castelletti, Nausheen W. Sadiq, Diane Beauchemin

Bibliographic record

VenueEncyclopedia of Analytical Chemistry · 2020
Typeother
Languageen
FieldChemistry
TopicAnalytical chemistry methods development
Canadian institutionsQueen's University
Fundersnot available
KeywordsInductively coupled plasma mass spectrometryMass spectrometryChemistryChromatographySample preparationEnvironmental chemistryEnvironmental analysisVaporizationInductively coupled plasmaContaminationGas chromatographyMatrix (chemical analysis)Analytical Chemistry (journal)Plasma

Abstract

fetched live from OpenAlex

Abstract The analysis of environmental samples is widely carried out to determine if a soil is safe for agricultural use, if water is safe to drink, if the air that we breathe can make us sick, how far reaching is pollution, if a contaminated site has been suitably remediated, etc. This article discusses how inductively coupled plasma mass spectrometry (ICPMS) can be used to this end. Indeed, with detection limits at the parts per trillion or even parts per quadrillion level, depending on the element and the instrument, ICPMS is very advantageous for the detection and quantification of toxic or potentially toxic species in environmental samples. This article describes sample preparation for ICPMS analysis and instrument calibration to yield accurate quantitative results. This includes the precautions that are often required, which vary depending on the type of analysis, sample matrix, instrument, and elements to be determined. It also includes techniques that can be coupled to ICPMS to increase its capabilities, such as laser ablation or electrothermal vaporization for direct solid analysis and liquid chromatography, gas chromatography, or capillary electrophoresis for speciation analysis, as speciation information is lost in the inductively coupled plasma (ICP) where all compounds are atomized.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Other · Consensus signal: Other
Teacher disagreement score0.178
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.001
Meta-epidemiology (broad)0.0020.001
Bibliometrics0.0000.001
Science and technology studies0.0000.001
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0220.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.027
GPT teacher head0.263
Teacher spread0.237 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreOther

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2020
Admission routes1
Has abstractyes

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