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Effect of the Composition of Additive Ash on the Thermal Behavior of Petroleum Coke Ash during Gasification

2020· article· en· W3082745519 on OpenAlexaff
Wei Li, Ben Wang, Jun Nie, Wu Yang, Lushi Sun, Deepak Pudasainee, Rajender Gupta

Bibliographic record

VenueEnergy & Fuels · 2020
Typearticle
Languageen
FieldEngineering
TopicIron and Steelmaking Processes
Canadian institutionsUniversity of Alberta
FundersMinistry of Science and Technology of the People's Republic of ChinaNational Natural Science Foundation of China
KeywordsReducing atmosphereMelting pointPetroleum cokeSlag (welding)Chemical engineeringMineralComposition (language)CokeMaterials scienceMetallurgyMelting temperatureFly ashAtmosphere (unit)ChemistryMineralogyThermodynamicsComposite material

Abstract

fetched live from OpenAlex

The behavior of ash fusion at high temperatures plays a key role in the stable operation of gasifiers. This study investigated the effect of synthetic mineral compounds on the transformation and ash fusion temperatures (AFTs) of petroleum coke (petcoke) ash in a steam atmosphere with the variation of the SiO 2 /Al 2 O 3 (Si/Al), Fe 2 O 3 /CaO (Fe/Ca), and V 2 O 5 /NiO (V/Ni) ratios and temperature. Thermodynamic equilibrium calculation was also applied to simulate the ash-melting process in petcoke gasification. The results show that the dominant crystalline phases in petcoke ash at high temperature are CaAl 2 Si 2 O 8, FeAl 2 O 4, and FeV 2 O 4 . The increase of temperature is conducive to the formation of low-melting minerals, such as, CaAl 2 Si 2 O 8 and FeAl 2 O 4 . High Si/Al is beneficial for the reduction of AFTs because high melting point minerals partly convert into slag and the low melting point mineral phase of CaAl 2 Si 2 O 8 transforms largely into slag. AFTs could be reduced at an Fe/Ca ratio of 0.5 when the content of slag in the ash reaches maximum and there are plenty of the low-melting minerals (CaAl 2 Si 2 O 8 ). A high V/Ni ratio was not conducive to the suppression of AFTs. The effect of Si/Al and Fe/Ca could effectively improve the AFTs of petcoke ash. A high ratio of Si/Al and the ratio of Fe/Ca at 0.5 were beneficial to the ash fusibility. AFTs under gasification atmosphere conditions have been predicted by FactSage.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.007
GPT teacher head0.202
Teacher spread0.195 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations11
Published2020
Admission routes1
Has abstractyes

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