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Deposition of Polychlorinated Biphenyls to Firn and Ice Cores at Opposite Polar Sites: Site M, Dronning Maud Land, Antarctica, and Holtedahlfonna, Svalbard

2020· article· en· W3096081974 on OpenAlexaff
Mark H. Hermanson, Elisabeth Isaksson, Richard Hann, Camilla Teixeira, Derek C. G. Muir

Bibliographic record

VenueACS Earth and Space Chemistry · 2020
Typearticle
Languageen
FieldEnvironmental Science
TopicToxic Organic Pollutants Impact
Canadian institutionsEnvironment and Climate Change Canada
Fundersnot available
KeywordsFirnIce coreGlacierGeologyIce capsDeposition (geology)PolarFlux (metallurgy)OceanographyPhysical geographyPolychlorinated biphenylAtmospheric sciencesEnvironmental scienceGeomorphologyGeographyEnvironmental chemistryChemistrySediment

Abstract

fetched live from OpenAlex

Firn and ice cores from glaciers and ice sheets at polar opposite locations, Site M, Dronning Maud Land, East Antarctica (lat 75.00 S, long. 15.00 E), and Holtedahlfonna, Svalbard (lat 79.13 N, long. 13.27 E), were analyzed for 81 polychlorinated biphenyl (PCB) congeners in 75 chromatographic peaks. Both sites are remote at high elevations and receive contaminant inputs from long-range atmospheric transport (LRAT). Firn cores from Site M formed one sample covering 1958–2000, while the Holtedahlfonna site has a historic record in 6 samples from 1953 to 2005. Most congeners at both sites are in triCB, tetraCB, and pentaCB homologs, and at Site M, these comprise 89% of PCB and 83% at Holtedahlfonna (with variability over time). Site M PCBs are dominated by pentaCB (48%), while Holtedahlfonna (whole-core average) is dominated by tetraCB (45%). The dominant congeners in triCB through hexaCB homologs are the same at both sites (PCB-28 + 31, PCB-70, PCB-101, PCB-138). The total PCB flux at Site M (4.1 pg cm–2 yr–1) was ∼33% of Holtedahlfonna (12.7 pg cm–2 yr–1) over whole-core history, perhaps resulting from high UV during spring Antarctic stratospheric ozone depletion leading to PCB decomposition. LRAT frequency diagrams showed a limited range of sources to Site M, leading to a hypothesis about transport through the stratosphere. The LRAT diagram for Holtedahlfonna shows greater than 1% time-coverage areas through central and northern Europe and Russia over 52 years. There is no apparent quantitative trend to PCB deposition over time at Holtedahlfonna, similar to observations elsewhere in the Arctic.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.115
Threshold uncertainty score0.744

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.207
Teacher spread0.197 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations3
Published2020
Admission routes1
Has abstractyes

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