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Record W3097231828 · doi:10.1021/acssuschemeng.0c07390

Physicochemical Characterization and Kinetic Modeling Concerning Combustion of Waste Berry Pomace

2020· article· en· W3097231828 on OpenAlexfundno aff
Ahmed I. Osman, Thomas J. Young, Charlie Farrell, John Harrison, Ala’a H. Al‐Muhtaseb, David W. Rooney

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2020
Typearticle
Languageen
FieldEngineering
TopicThermochemical Biomass Conversion Processes
Canadian institutionsnot available
FundersCore Research for Evolutional Science and TechnologyBryden Centre, Queen's University BelfastEngineering and Physical Sciences Research CouncilInterregEuropean CommissionQueen's UniversityQueen's University BelfastDepartment for the Economy
KeywordsPomaceActivation energyCombustionIsothermal processKinetic energyReaction rate constantChemistryDifferential scanning calorimetryOrder of reactionThermodynamicsReaction rateMaterials scienceAtmospheric temperature rangeKineticsAnalytical Chemistry (journal)Physical chemistryOrganic chemistryCatalysis

Abstract

fetched live from OpenAlex

Herein waste biomass (blackberry pomace) was physicochemically characterized along with its thermochemical products. This is coupled with the evaluation of the kinetic triplet (activation energy, pre-exponential constant, and the rate of reaction) and thermal predictions for the combustion process for the first time via the AKTS thermokinetics package. The main kinetic modeling method employed was the differential isoconversional analysis; however, the Flynn–Wall–Ozawa and ASTM E-698 methods were used as comparisons. The model was developed and validated from experimental DSC and TGA data, resulting in an excellent match (R2 = 0.99544 and 0.99194, respectively). The activation energies were evaluated using the ASTM-E698 method (88.64 kJ mol–1) and Flynn–Wall–Ozawa methods (50–140 kJ mol–1). The differential isoconversional method showed that activation energy values were in the range of 84–197 kJ mol–1 for the combustion of berry pomace. Isothermal predictions based on the model were indicated at temperatures of 560 and 600 °C; the reaction had achieved 100% completion (α = 1) after 30 and 6 min, respectively. For the nonisothermal prediction, the heating rates of 50, 75, and 100 °C/min have a two-stage rate profile with a maximum peak in the first stage of the reaction. Thereafter, the reaction rate increases once again but not to the same effect as the first initial stage. For instance, at 100 °C/min, stages 1 and 2 are reported as 0.005381 and 0.005148 s–1,respectively. Overall, this study demonstrates the success of the approach in modeling the thermochemical conversion of berry pomace as waste stream biomass.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.193
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.174
Teacher spread0.167 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations47
Published2020
Admission routes1
Has abstractyes

Explore more

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