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Record W3099688525 · doi:10.1002/ente.202000791

All‐Ambient‐Processed CuSCN as an Inexpensive Alternative to Spiro‐OMeTAD for Perovskite‐Based Devices

2020· article· en· W3099688525 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.

Bibliographic record

VenueEnergy Technology · 2020
Typearticle
Languageen
FieldEngineering
TopicPerovskite Materials and Applications
Canadian institutionsÉcole de Technologie SupérieureInstitut National de la Recherche Scientifique
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsFabricationMaterials sciencePhotodetectorPerovskite (structure)OptoelectronicsDopantNanotechnologyEnergy conversion efficiencyDopingChemical engineering

Abstract

fetched live from OpenAlex

Organic hole‐transporting materials (HTM) are widely used for high‐efficiency solar cells. However, compared with their inorganic counterparts, these materials are often expensive and require complex synthesis methods and the addition of costly dopants to improve their performance. In addition, exposure to the ambient environment affects the chemical stability of some organic materials as well as their device characteristics. Herein, an all‐ambient fabrication method is used to develop a CuSCN layer as an alternative to the conventional Spiro‐OMeTAD HTM. CuSCN thin films are incorporated into both solar cells and photodetectors to study their effect on the optoelectronic properties of these devices. For the solar cells made with CuSCN, a power conversion efficiency of 14.3% is achieved, with remarkable ambient‐stability without encapsulation. Regarding the photodetectors with CuSCN, high‐specific detectivity up to 10 12 Jones is exhibited. Solution‐processed devices exhibit overall impressive performances and represent an essential step toward large‐scale fabrication of efficient, stable, facile, and inexpensive perovskite‐based optoelectronic technologies.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.295
Threshold uncertainty score0.907

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.021
GPT teacher head0.267
Teacher spread0.246 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it