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Record W3101521471 · doi:10.1002/cjce.23943

Diethylenetriamine as a selective pyrrhotite depressant: Properties, application, and mitigation strategies

2020· article· en· W3101521471 on OpenAlexafffundvenueabout
Erin Furnell, Xinyi Tian, Erin R. Bobicki

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2020
Typearticle
Languageen
FieldEngineering
TopicMetal Extraction and Bioleaching
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of Canada
KeywordsTailingsDiethylenetriamineChelationPyrrhotiteEffluentLimeChemistrySmeltingEnvironmental chemistryMetallurgyEnvironmental scienceMaterials scienceMineralogyInorganic chemistryEnvironmental engineeringOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Pyrrhotite (Po) is an abundant iron sulphide mineral that occurs in nickel sulphide deposits, such as those in Sudbury, Ontario. Due to its low economic value and its high contribution to SO 2 emissions produced during smelting, Po is rejected into the tailings during mineral processing. The rejection of Po can be accomplished in several ways, including by using chelating agents such as diethylenetriamine (DETA) as depressants in froth flotation. DETA can significantly improve nickel recovery and concentrate grades; however, it is challenging to manage in the tailings area. DETA, when used, forms stable chelates with Ni 2+ and Cu 2+ which cannot be precipitated with traditional lime treatment. Once in the tailings management area, DETA can desorb from Po solids upon dilution or with changes in temperature and/or pH. The species chelated with DETA can also change depending on the availability of the ions in solution. The use of DETA can, therefore, lead to concentrations of Ni 2+ and Cu 2+ in final effluent that exceed the regulated amounts. Due to the challenges with chelated metals in effluent, it is recommended that the chelating agents be removed from the tailings stream before it is deposited. Although DETA‐metal chelates are rarely discussed in the literature, some mitigation and degradation strategies investigated by industry are discussed in this review. DETA degradation methods are also discussed, with the primary focus being on biodegradation. DETA has generally been described as recalcitrant to biodegradation although there is evidence that proper acclimation should allow bacteria to develop DETA degradation pathways.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.277
Threshold uncertainty score0.276

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.009
GPT teacher head0.178
Teacher spread0.169 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations13
Published2020
Admission routes4
Has abstractyes

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