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Record W3102447218

EXCITATION OF THE AROMATIC INFRARED EMISSION BANDS: CHEMICAL ENERGY IN HYDROGENATED AMORPHOUS CARBON PARTICLES?

2011· article· en· W3102447218 on OpenAlexaff

Bibliographic record

VenueUCL Discovery (University College London) · 2011
Typearticle
Languageen
FieldPhysics and Astronomy
TopicAstrophysics and Star Formation Studies
Canadian institutionsUniversity of Waterloo
Fundersnot available
KeywordsDangling bondExcitationAmorphous carbonInfraredMoleculeCarbon fibersMaterials scienceWavelengthAmorphous solidChemical energyChemical physicsAtomic physicsAnalytical Chemistry (journal)PhotochemistryChemistryOptoelectronicsOpticsOrganic chemistryPhysicsComposite material
DOInot available

Abstract

fetched live from OpenAlex

We outline a model for the heating of hydrogenated amorphous carbon (HAC) dust via the release of stored chemical energy and show that this energy (similar to 12 kJ mole(-1)) is sufficient to heat dust grains of classical size (50-1000 angstrom) to temperatures at which they can emit at 3.3 mu m and other "UIR" wavelengths. Using laboratory data, we show that this heating process is consistent with a concentration of a few percent of dangling bonds in HAC and may be initiated by the recombination of trapped H atoms. We suggest that the release of chemical energy from dust represents an additional source of excitation for the UIR bands relaxing the previous requirement that only stochastically heated molecules having fewer than similar to 50 atoms can produce emission at 3.3 mu m.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Theoretical or conceptual · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.316
Threshold uncertainty score0.395

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.008
GPT teacher head0.167
Teacher spread0.159 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designTheoretical or conceptual
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations34
Published2011
Admission routes1
Has abstractyes

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