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Record W3122246534 · doi:10.22215/etd/2016-11617

Development of a Tunable Diode Laser Absorption Spectroscopy Mass-Flux Sensor for Quantifying Hydrocarbon Storage Tank Venting

2016· dissertation· en· W3122246534 on OpenAlexaff
Simon A. Festa-Bianchet

Bibliographic record

Venuenot available
Typedissertation
Languageen
FieldChemistry
TopicSpectroscopy and Laser Applications
Canadian institutionsCarleton University
Fundersnot available
KeywordsTunable diode laser absorption spectroscopyAbsorption (acoustics)Flux (metallurgy)SpectroscopyStorage tankMaterials scienceAbsorption spectroscopyEnvironmental scienceLaserHydrocarbonAnalytical Chemistry (journal)DiodeMass spectrometryWavelengthOpticsTunable laserOptoelectronicsChemistryWaste managementEngineeringPhysicsEnvironmental chemistryChromatography

Abstract

fetched live from OpenAlex

Fixed-roof liquid hydrocarbon storage tanks are a recognized source of volatile organic compounds and greenhouse gases.However, current emissions estimates suffer from a lack of reliable models due to poor in situ validation.This work presents the development and characterization of an intrinsically safe, low velocity mass-flux sensor for monitoring storage tank venting.The sensor is based on tunable diode laser absorption spectroscopy (TDLAS) with wavelength modulation.Similar sensors have been successfully used to measure high velocity flows, such as shock propagation and scramjet combustor exhaust.The oxygen within the vapour space of fixed-roof storage tanks is targeted in the near-IR as the absorption species.Sensor design, optimum operational parameters, and indoor characterization results are presented.An oxygen concentration precision of greater than 0.11% absolute was achieved over the tested range of 2.5 to 21% O2.For measurements at 21% O2, a velocity standard deviation of 0.24 m/s for 30-s average measurements was achieved, which could be improved to 0.07 m/s with a 10-minute interval drift correction.However, the velocity measurement accuracy was poor at lower O2 concentrations, restricting the mass flux capability of the current system.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Methods · Consensus signal: none
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0010.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.025
GPT teacher head0.304
Teacher spread0.279 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreMethods

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2016
Admission routes1
Has abstractyes

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