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Record W3126403336 · doi:10.1002/agt2.29

Enhancing photovoltaic performance via aggregation dynamics control in fused‐ring electron acceptor

2021· article· en· W3126403336 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueAggregate · 2021
Typearticle
Languageen
FieldEngineering
TopicOrganic Electronics and Photovoltaics
Canadian institutionsMinistry of Education and Child Care
FundersNational Natural Science Foundation of China
KeywordsPhotocurrentMaterials scienceCrystallinityShort circuitAcceptorEnergy conversion efficiencyElectron acceptorAbsorption (acoustics)HOMO/LUMOElectron mobilityChemical physicsOptoelectronicsPhotochemistryChemistryVoltageOrganic chemistryComposite materialMoleculePhysics

Abstract

fetched live from OpenAlex

Abstract A new fused‐ring electron acceptor FNIC3 with dynamics controlled aggregation behavior was synthesized. FNIC3 shows strong absorption in 600–900 nm, HOMO/LUMO energy levels of −5.59/−4.04 eV, and electron mobility of 1.2 × 10 −3 cm 2 V −1 s −1 . The aggregation of FNIC3 shows strong dependency on film formation time. Prolongation of film formation time promotes the crystallization of FNIC3, leading to improved crystallinity and enlarged aggregate sizes. Aggregation of FNIC3 significantly influences the photovoltaic device parameters. Appropriate aggregation red‐shifts the absorption and improves the mobilities of the blend, which contributes to high photocurrent and fill factor thus high power conversion efficiency (PCE). Overaggregation leads to increased nonradiative energy loss and insufficient charge generation, resulting in decreased open‐circuit voltage and short‐circuit current density. The blends based on PM6:FNIC3 fabricated under proper film formation time exhibit a PCE of 12.3%, higher than those fabricated under short and long film formation time (10.0–10.5%).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.300
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.003
GPT teacher head0.188
Teacher spread0.185 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it