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Record W3128963167 · doi:10.1002/ejic.202001117

Chromic Platinum Complexes Containing Multidentate Ligands

2021· article· en· W3128963167 on OpenAlexafffund
Miguel A. Soto, Raksha Kandel, Mark J. MacLachlan

Bibliographic record

VenueEuropean Journal of Inorganic Chemistry · 2021
Typearticle
Languageen
FieldMaterials Science
TopicPhotochromic and Fluorescence Chemistry
Canadian institutionsUniversity of British Columbia
FundersNatural Sciences and Engineering Research Council of CanadaUniversity of British Columbia
KeywordsChemistryDenticityPlatinumLigand (biochemistry)Transition metalLuminescenceMetalPhotochemistryRutheniumCrystallographyCharge (physics)OptoelectronicsCatalysisOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Platinum(II) complexes display versatile chromic behavior as a consequence of their square planar geometry, which enables intra‐ and intermolecular Pt⋅⋅⋅Pt interactions via open axial coordination sites. These metallophilic interactions are known to generate metal‐metal‐to‐ligand‐charge transfer (MMLCT) transitions, in addition to the ligand‐to‐ligand charge transfer (LLCT) and metal‐to‐ligand‐charge‐transfer (MLCT) transitions that are already present. The electronic properties of such complexes, and consequently the magnitude and intensity of these transitions, can be modulated by various functional groups as well as environmental factors, affording control over the color and luminescence. The responsive behavior of these complexes makes them attractive candidates for chromic devices with applications in memory, encryption, sensors, and optoelectronics. This Minireview summarizes the mechanisms and reversibility of optical chromism in platinum(II) complexes, with a focus on the recent developments in the literature.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.004
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.013
GPT teacher head0.228
Teacher spread0.215 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations51
Published2021
Admission routes2
Has abstractyes

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