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Record W3137454749 · doi:10.1021/acssuschemeng.0c08692

Natural Emulgel from Dialdehyde Cellulose for Lipophilic Drug Delivery

2021· article· en· W3137454749 on OpenAlexafffund
Roya Koshani, Mandana Tavakolian, Theo G. M. van de Ven

Bibliographic record

VenueACS Sustainable Chemistry & Engineering · 2021
Typearticle
Languageen
FieldMaterials Science
TopicPickering emulsions and particle stabilization
Canadian institutionsMcGill University
FundersFonds de recherche du Québec – Nature et technologiesNatural Sciences and Engineering Research Council of Canada
KeywordsChitosanEmulsionChemistryPulmonary surfactantFourier transform infrared spectroscopyCelluloseAmine gas treatingDrug deliveryNuclear chemistrySonicationChemical engineeringOrganic chemistryMaterials sciencePolymer chemistryChromatographyBiochemistry

Abstract

fetched live from OpenAlex

In this study, we develop a cellulosic emulgel based on dialdehyde cellulose (DAC) cross-linked with chitosan using an embedded emulsion for the delivery of lipophilic compounds. First, a surfactant-free oil-in-water emulsion was prepared by ultrasonication, using DAC as an interfacial stabilizer. Then, by adding chitosan to the emulsion, the aldehyde groups of DAC chemically reacted with the amine groups of chitosan via a Schiff base reaction to form a cross-linked emulgel, which was confirmed by nuclear magnetic resonance and Fourier transform infrared spectroscopy. The developed emulgel with a larger surface area (∼81 m2 g–1) swells more slowly compared to its hydrogel homologue (∼5 m2 g–1). Scanning electron microscopy imaging along with Barrett, Joyner and Halenda method results indicated the formation of a homogenized structural matrix of micro- and nanosized pores. β-Carotene was loaded in the oil phase, and its release was measured using a static orogastrointestinal method. It was shown that after safely passing the oral processing, only ∼20% of β-carotene is released in the stomach, while a gradual increase in β-carotene release, up to 50%, is observed during a 4-h stay in the intestines. This emulgel, rationally processed via safe and green strategies, is a promising candidate for the delivery of lipophilic compounds, specifically for the purpose of oral administration.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.017
Threshold uncertainty score0.823

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.195
Teacher spread0.191 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations46
Published2021
Admission routes2
Has abstractyes

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