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Record W3138892600 · doi:10.1002/cjce.24110

Mechanism and kinetics study of Mg <sup>2+</sup> removal from wet‐process phosphoric acid by Sinco‐430 resin

2021· article· en· W3138892600 on OpenAlexvenueno aff
Chao Hu, Xuefang Yan, Run Zhou Ye, Yanjun Zhong, Haozhou Liu, Xin-Long Wang, Lin Yang

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicAdsorption and biosorption for pollutant removal
Canadian institutionsnot available
Fundersnot available
KeywordsPhosphoric acidActivation energyIon-exchange resinChemistryKineticsDiffusionFourier transform infrared spectroscopyNuclear chemistryKinetic energyX-ray photoelectron spectroscopyReaction mechanismAnalytical Chemistry (journal)Ion exchangeChemical kineticsIonCatalysisChromatographyInorganic chemistryPhysical chemistryChemical engineeringOrganic chemistryThermodynamics

Abstract

fetched live from OpenAlex

Abstract The reaction mechanism and kinetics of Sinco‐430 cation exchange resin removing Mg 2+ from wet‐process phosphoric acid (WPA) were studied. Fourier transform infrared and X‐ray photoelectron spectroscopy analyses revealed that the main functional group of the resin that combined with Mg 2+ ions was –SO 3 H. To investigate the most suitable conditions for Mg 2+ removal, the operating parameters that could affect Mg 2+ removal were studied. The results demonstrated that under optimal conditions (T = 50°C, solid to liquid mass ratio = 0.3, and P 2 O 5 content = 20 wt.%) the reaction reached equilibrium in 8 min and Mg 2+ removal rate reached 59.09%. The kinetic model and activation energy of the reaction were second‐order and 19.11 kJ/mol according to kinetic analysis, respectively. The diffusion model of Mg 2+ removal was determined as pore diffusion according to the comparison of three different diffusion models. H 3 PO 4 was recovered using deionized water and Mg 2+ was removed from the loading resin with 20 wt.% H 2 SO 4 . In addition, after eight loading/regeneration cycles, the Mg 2+ removal ability of the Sinco‐430 resin remained the same. The Mg 2+ removal rate in a fixed‐bed reactor was 98.83%, higher than that obtained in a continuous stirred‐tank reactor.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.003

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.184
Teacher spread0.178 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations5
Published2021
Admission routes1
Has abstractyes

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Same venueThe Canadian Journal of Chemical EngineeringSame topicAdsorption and biosorption for pollutant removalFrench-language works237,207