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Record W3155012853

Surface Enhanced Raman Spectroscopy (SERS) Detection of β-Estradiol in Milk by Molecularly Imprinted Polymers on Biogenic Silica and Silver Nanoparticles

2017· article· en· W3155012853 on OpenAlexaff
Weihao Lu, Samuel M. Mugo

Bibliographic record

VenueStudent Research Proceedings · 2017
Typearticle
Languageen
FieldChemistry
TopicDye analysis and toxicity
Canadian institutionsMacEwan University
Fundersnot available
KeywordsEthylene glycol dimethacrylateSilver nanoparticleMolecularly imprinted polymerPolymerizationMethacrylic acidNanoparticleMaterials scienceRaman spectroscopyMonomerPrecipitation polymerizationDetection limitPolymerEthylene glycolChemical engineeringPolymer chemistryChemistryNuclear chemistryNanotechnologyOrganic chemistrySelectivityRadical polymerizationChromatographyCatalysis
DOInot available

Abstract

fetched live from OpenAlex

The highly sensitive surfaced-enhanced Raman spectroscopy (SERS) and the directive selection of molecularly imprinted polymers (MIP) provided a simple and rapid method to detect the content of β-estradiol in milk sample which exists in low concentration at natural level. The MIPs were synthesized by surface polymerization of β-estradiol (template), methacrylic acid (the monomer), and ethylene glycol dimethacrylate (cross-linking agent), with 4,4’ azobis (4-cyanopentanoyl) chloride initiator covalently grafted on the biogenic silica surface.  The NIPs were also synthesized in a similar version to  MIPs, but polymerization done  without β-estradiol template. The surface morphology of MIPs and NIPs by scanning electron microscopy (SEM) showed a clear difference on their structures. Silver and silica nanoparticles were served as SERS active substrates for signal enhancement. The limit of detection (LOD) for MIPs-silver nanoparticles  was 1.0  ppm, whereas for MIPs-silica, the LOD was 0.78 ppm. As the result, biogenic silica nanoparticles gave a more enhanced Raman signal compared to the conventional silver nanoparticles. Discipline: Chemistry Faculty Mentor: Dr. Samuel Mugo

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.001
Threshold uncertainty score0.002

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.363
Teacher spread0.330 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2017
Admission routes1
Has abstractyes

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