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Record W3155012853

Surface Enhanced Raman Spectroscopy (SERS) Detection of β-Estradiol in Milk by Molecularly Imprinted Polymers on Biogenic Silica and Silver Nanoparticles

2017· article· en· W3155012853 on OpenAlex
Weihao Lu, Samuel M. Mugo

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueStudent Research Proceedings · 2017
Typearticle
Languageen
FieldChemistry
TopicDye analysis and toxicity
Canadian institutionsMacEwan University
Fundersnot available
KeywordsEthylene glycol dimethacrylateSilver nanoparticleMolecularly imprinted polymerPolymerizationMethacrylic acidNanoparticleMaterials scienceRaman spectroscopyMonomerPrecipitation polymerizationDetection limitPolymerEthylene glycolChemical engineeringPolymer chemistryChemistryNuclear chemistryNanotechnologyOrganic chemistrySelectivityRadical polymerizationChromatographyCatalysis
DOInot available

Abstract

fetched live from OpenAlex

The highly sensitive surfaced-enhanced Raman spectroscopy (SERS) and the directive selection of molecularly imprinted polymers (MIP) provided a simple and rapid method to detect the content of β-estradiol in milk sample which exists in low concentration at natural level. The MIPs were synthesized by surface polymerization of β-estradiol (template), methacrylic acid (the monomer), and ethylene glycol dimethacrylate (cross-linking agent), with 4,4’ azobis (4-cyanopentanoyl) chloride initiator covalently grafted on the biogenic silica surface.  The NIPs were also synthesized in a similar version to  MIPs, but polymerization done  without β-estradiol template. The surface morphology of MIPs and NIPs by scanning electron microscopy (SEM) showed a clear difference on their structures. Silver and silica nanoparticles were served as SERS active substrates for signal enhancement. The limit of detection (LOD) for MIPs-silver nanoparticles  was 1.0  ppm, whereas for MIPs-silica, the LOD was 0.78 ppm. As the result, biogenic silica nanoparticles gave a more enhanced Raman signal compared to the conventional silver nanoparticles. Discipline: Chemistry Faculty Mentor: Dr. Samuel Mugo

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.005
Threshold uncertainty score0.685

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.033
GPT teacher head0.363
Teacher spread0.330 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it