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Record W3156828228 · doi:10.1002/cjce.24135

Simultaneous removal of elemental mercury and <scp>NO</scp> from flue gas by the <scp> CeO <sub>2</sub> </scp> / <scp> TiO <sub>2</sub> </scp> catalysts and the mechanism investigation

2021· article· en· W3156828228 on OpenAlexvenueno aff
Zhong He, Yifei Long, Wenjie Liu, Xiaoyi Li, Yuan Wang, Jiangjun Hu

Bibliographic record

VenueThe Canadian Journal of Chemical Engineering · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicMercury impact and mitigation studies
Canadian institutionsnot available
Fundersnot available
KeywordsFlue gasCatalysisAdsorptionChemistryMercury (programming language)OxygenChemical engineeringInorganic chemistrySpecific surface areaNitrogenOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Mercury pollution has become one of the high‐profile environmental problems in the world. A series of Ce y Ti catalyst were synthesized by sol–gel method, and the process of simultaneous conversion of NO and removal of mercury (Hg 0 ) in the flue gas was studied. BET, SEM, and XRD were used to systematically detect the physicochemical properties of the catalysts, which show that excessive Ce loading would make its specific surface area reduce. The NO conversion efficiency would increase with the increase of the Ce loading. The optimal Ce/Ti mass ratio was 0.3. A part of the adsorbed NO would be oxidized by the active oxygen species on the catalyst surface to produce a certain amount of nitrogen‐containing substances, such as NO + , NO 3− , or NO 2 . The produced substances could promote the adsorption and oxidation of Hg 0 . The NO conversion was very dependent on the oxygen in the flue gas. The activity of the Ce 0.3 Ti catalyst was promoted in the presence of O 2 . SO 2 and H 2 O would inhibit the reaction of NO conversion and Hg 0 removal. The mechanisms of the catalytic system have been proved via the Mars‐Maessen mechanism.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.002
Threshold uncertainty score0.004

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.177
Teacher spread0.172 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations1
Published2021
Admission routes1
Has abstractyes

Explore more

Same venueThe Canadian Journal of Chemical Engineering→Same topicMercury impact and mitigation studies→French-language works237,207→