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Record W3157138328 · doi:10.3389/fclim.2021.656108

Scaling CO2 Capture With Downstream Flow CO2 Conversion to Ethanol

2021· article· en· W3157138328 on OpenAlexfundaboutno aff
Grant Pace, Stafford W. Sheehan

Bibliographic record

VenueFrontiers in Climate · 2021
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsnot available
FundersCanada's Oil Sands Innovation AllianceOntario Centre of InnovationNew York State Energy Research and Development AuthorityOntario Centres of ExcellenceNational Aeronautics and Space Administration
KeywordsDownstream (manufacturing)Greenhouse gasEnvironmental scienceScale (ratio)ScalingRaw materialProcess engineeringMaterial flow analysisWaste managementEnvironmental economicsEngineeringChemistryOperations management

Abstract

fetched live from OpenAlex

To prevent the global average temperature from increasing more than 1.5°C and lower the concentration of greenhouse gases (GHGs) in the atmosphere, most emissions trajectories necessitate the implementation of strategies that include both GHG mitigation and negative emissions technologies (NETs). For NETs, there are unique research challenges faced by both CO 2 capture and utilization to scale in an economically feasible manner. Starting with incumbent methods, wherein CO 2 is recovered from a high concentration source, and moving toward CO 2 capture from more widely available dilute sources, we outline how CO 2 capture systems interface with downstream utilization in flow reactors. To provide a real-world point of comparison, we analyze CO 2 sourcing for Air Company's CO 2 -to-alcohols pilot and demonstration scale deployments in Brooklyn, New York, USA and Calgary, Alberta, Canada as case studies. The degree of reduction in atmospheric CO 2 depends on product alcohol usage; for example, use as a fixed chemical feedstock provides longer term emissions reduction than as a fuel, which is eventually oxidized. Lastly, we discuss the barriers that are present for economic scale-up of CO 2 capture and utilization technologies broadly.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.001
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.025
Threshold uncertainty score0.050

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.001
Meta-epidemiology (narrow)0.0010.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0010.001
Open science0.0010.001
Research integrity0.0010.001
Insufficient payload (model declined to judge)0.0030.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.194
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2021
Admission routes2
Has abstractyes

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Same venueFrontiers in ClimateSame topicCarbon Dioxide Capture TechnologiesFrench-language works237,207