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Record W3157138328 · doi:10.3389/fclim.2021.656108

Scaling CO2 Capture With Downstream Flow CO2 Conversion to Ethanol

2021· article· en· W3157138328 on OpenAlexfundaboutno aff
Grant Pace, Stafford W. Sheehan

Bibliographic record

VenueFrontiers in Climate · 2021
Typearticle
Languageen
FieldEngineering
TopicCarbon Dioxide Capture Technologies
Canadian institutionsnot available
FundersCanada's Oil Sands Innovation AllianceOntario Centre of InnovationNew York State Energy Research and Development AuthorityOntario Centres of ExcellenceNational Aeronautics and Space Administration
KeywordsDownstream (manufacturing)Greenhouse gasEnvironmental scienceScale (ratio)ScalingRaw materialProcess engineeringMaterial flow analysisWaste managementEnvironmental economicsEngineeringChemistryOperations management

Abstract

fetched live from OpenAlex

To prevent the global average temperature from increasing more than 1.5°C and lower the concentration of greenhouse gases (GHGs) in the atmosphere, most emissions trajectories necessitate the implementation of strategies that include both GHG mitigation and negative emissions technologies (NETs). For NETs, there are unique research challenges faced by both CO 2 capture and utilization to scale in an economically feasible manner. Starting with incumbent methods, wherein CO 2 is recovered from a high concentration source, and moving toward CO 2 capture from more widely available dilute sources, we outline how CO 2 capture systems interface with downstream utilization in flow reactors. To provide a real-world point of comparison, we analyze CO 2 sourcing for Air Company's CO 2 -to-alcohols pilot and demonstration scale deployments in Brooklyn, New York, USA and Calgary, Alberta, Canada as case studies. The degree of reduction in atmospheric CO 2 depends on product alcohol usage; for example, use as a fixed chemical feedstock provides longer term emissions reduction than as a fuel, which is eventually oxidized. Lastly, we discuss the barriers that are present for economic scale-up of CO 2 capture and utilization technologies broadly.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Simulation or modeling · Consensus signal: none
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.669
Threshold uncertainty score0.940

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.006
GPT teacher head0.194
Teacher spread0.189 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designSimulation or modeling
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations12
Published2021
Admission routes2
Has abstractyes

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