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Record W3157184689 · doi:10.1088/2515-7620/abfa65

Atmospheric trace gas trends obtained from FTIR column measurements in Toronto, Canada from 2002-2019

2021· article· en· W3157184689 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.
fundA Canadian funder is recorded on the work.
aboutThe title or abstract carries a Canadian signal from the geographic lexicon.

Bibliographic record

VenueEnvironmental Research Communications · 2021
Typearticle
Languageen
FieldEnvironmental Science
TopicAtmospheric and Environmental Gas Dynamics
Canadian institutionsUniversity of Toronto
FundersNatural Sciences and Engineering Research Council of CanadaEnvironment and Climate Change Canada
KeywordsFourier transform infrared spectroscopyTrace gasAnalytical Chemistry (journal)TroposphereAtmospheric chemistryChemistryAtmospheric sciencesPhysicsEnvironmental chemistryOzoneOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Total columns of C 2 H 2 , C 2 H 6 , CH 4 , CH 3 OH, CO, H 2 CO, HCl, HCN, HCOOH, HF, HNO 3 , N 2 O, NH 3 and O 3 were retrieved from 2002-2019 using a Fourier transform infrared (FTIR) spectrometer at the University of Toronto Atmospheric Observatory (TAO). Trends and enhancement events were determined by fitting trended Fourier series, and bootstrapping was used to identify the statistical significance. Trends from 2002 to 2019 (%/year, with 2 σ uncertainties) were found for C 2 H 2 (−1.12 ± 0.30), C 2 H 6 (−0.74 ± 0.73 from 2002–2008 and 1.19 ± 0.27 from 2009–2019), CH 4 (0.26 ± 0.10 from 2002–2008 and 0.41 ± 0.03 from 2009–2019), CO (−0.90 ± 0.07), HCN (−0.51 ± 0.21), HCOOH (−2.15 ± 0.64), HF (0.59 ± 0.11), HNO 3 (0.36 ± 0.13), N 2 O (0.28 ± 0.02), NH 3 (3.56 ± 0.85), and O 3 (0.28 ± 0.19 and −0.05 ± 0.07 for tropospheric and stratospheric columns, respectively). The GEOS-Chem chemical transport model showed that wetland emissions were the largest contributor to CH 4 columns measured at TAO (average relative contribution of 31.7%), and that CH 4 oxidation was a major source of CO (accounting for 30.9%).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.098
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.001
Science and technology studies0.0010.001
Scholarly communication0.0000.000
Open science0.0020.002
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0440.001

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.036
GPT teacher head0.294
Teacher spread0.258 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it