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Record W3159529765

Nanoparticles for photodiagnosis and photodynamic therapy of malignant diseases

2009· preprint· en· W3159529765 on OpenAlexaff
Marie Ange d'Hallewin, Frédéric Marchal, François Guillemin, Lina Bezdetnaya

Bibliographic record

VenueHAL (Le Centre pour la Communication Scientifique Directe) · 2009
Typepreprint
Languageen
FieldChemistry
TopicClick Chemistry and Applications
Canadian institutionsCentre d'expertise et de recherche en infrastructures urbaines
Fundersnot available
KeywordsPhotodynamic therapyLiposomeFluorescenceChemistryBiophysicsPhotosensitizerReactive oxygen speciesDrug deliveryDrugQuenching (fluorescence)Cancer researchPhotochemistryPharmacologyMedicineBiochemistryBiologyOrganic chemistry
DOInot available

Abstract

fetched live from OpenAlex

Photodiagnosis as well as photodynamic therapy (PDT) are based on the use of a photosensitzer (PS) molecule that upon light illumination will either fluoresce or transfer energy to oxygen molecules to create reactive oxygen species that are highly cytotoxic. Since those molecules have a higher affinity towards malignant tissue, they can be used to either indicate the presence of cancer or to destroy it. The main problem with these techniques resides in the relative lack of specific uptake, resulting in false positive diagnosis, excessive tissue destruction and long standing cutaneous sensitization. Incorporation of PS into nanoparticle platforms aims to minimize those side effects, mainly due to the enhanced permeability retention effect and to enhance photodynamic activity due to monomerization of the active compound. Our group is actively investigating photophysical properties of different carrier systems as well as preclinical work to evaluate potential new diagnostic and therapeutic approaches. Liposomal formulations of mTHPC (Foscan®) have been investigated in collaboration with Biolitec AG. The PS was rapidly eliminated from the plasma and maximal therapeutic efficacy was observed when microscopic studies indicated presence of high drug doses in both endothelial cells and tumor cells. Intratumoral drug injections were tested in a model of breast cancer recurrence and revealed unusual features, namely progressive increase of fluorescence that was maximal 24 H after administration. This appeared to be due to a phenomenon of photoinduced fluorescence quenching due to energy transfer between PS molecules within the liposomes. We also developed a new approach for PDT, namely to apply illumination in order to prevent recurrence of bladder cancer following fluorescence guided transurethral resection. In order to avoid excessive photobleaching of the drug, we are currently investigating dendrimerized photosensitizers in collaboration with the University College of London. Those dendrimers appear to have a much higher affinity towards bladder cancer in vivo and to provide a sustained release and uptake of the active component. A third axis of our research is to visualize sentinel lymph nodes with quantum dots. Together with the EPCI (Industrial Physico-Chemical High School, Paris), we have defined the coating that offers the highest lymphotropicity in a newly developed model of metastatic breast cancer. We are currently investigating a new imaging tool to detect thoracic lymph nodes containing NIR emitting quantum dots

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.001
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.042
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0010.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0010.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.014
GPT teacher head0.245
Teacher spread0.230 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2009
Admission routes1
Has abstractyes

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