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Record W3164037333 · doi:10.1002/hyp.14248

Water recovery rate and isotopic signature of cryogenic vacuum extracted spiked soil water following oven‐drying at different temperatures

2021· article· en· W3164037333 on OpenAlexaff
Mingyi Wen, Bingcheng Si, Yanwei Lu, Hongxiu Wang

Bibliographic record

VenueHydrological Processes · 2021
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicGroundwater and Isotope Geochemistry
Canadian institutionsUniversity of Saskatchewan
FundersNational Natural Science Foundation of China
KeywordsSoil waterChemistryEnvironmental chemistryExtraction (chemistry)Isotope-ratio mass spectrometryStable isotope ratioBound waterIsotopeWater contentMass spectrometryEnvironmental scienceSoil scienceChromatographyGeology

Abstract

fetched live from OpenAlex

Abstract Extracting water from soils is often a critical step for obtaining soil water isotope information. Cryogenic vacuum extraction (CVE), the most widely used laboratory‐based removal technique, produces biased isotope composition and the mechanisms causing the biases remain uncertain. Here, we conducted spiking tests on soil samples oven‐dried at 105 and 205°C, respectively. The recovery rate and isotopic composition of the extracted water were analysed. Our results show that conventional oven‐drying (105°C) was not sufficient to liberate tightly bound water from soils but oven‐drying at temperatures above 205°C was. Part of the tightly bound water in soil was extracted by CVE, because the extraction capacity of CVE (heating at 95°C) was equivalent to oven‐drying at temperature between 105 and 205°C. Moreover, the two pretreatments yielded markedly differences in water recovery rates. And with increasing ratios of clay contents to water contents, the recovery rates of the pretreated soil at 105°C trended upward above 100%, but that of 205°C trended downward below 100%. Further, the 2 H and 18 O signatures of the extracted water from the soil pretreated at 205°C were both depleted relative to reference water, but the pretreatment at 105°C showed enriched 18 O and depleted 2 H. This suggests that oxygen isotope exchange may have occurred between tightly bound water and soil minerals, resulting in enriched 18 O in water for the 105°C pretreatments. For the 205°C pretreatment, pre‐existing soil water was completely removed and relative to spiking water, isotopic signatures of the extracted water followed equilibrium fractionation law due to incomplete extraction. Therefore, our results suggested that the biased isotopic signatures of water extracted by CVE may be partially due to incomplete extraction and mixture of added water with the residual tightly bound water that pre‐exists before spiking.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesInsufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.057
Threshold uncertainty score0.998

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.010
GPT teacher head0.193
Teacher spread0.183 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designBench or experimental
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations17
Published2021
Admission routes1
Has abstractyes

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