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Record W3176187916 · doi:10.1002/lno.11862

Dynamic changes in size‐fractionated dissolved organic matter composition in a seasonally ice‐covered Arctic River

2021· article· en· W3176187916 on OpenAlexaffabout
Hui Lin, Huacheng Xu, Yihua Cai, Claude Belzile, Robie W. Macdonald, Laodong Guo

Bibliographic record

VenueLimnology and Oceanography · 2021
Typearticle
Languageen
FieldEarth and Planetary Sciences
TopicMarine and coastal ecosystems
Canadian institutionsUniversity of ManitobaFisheries and Oceans CanadaUniversité du Québec à Rimouski
FundersUniversity of Wisconsin-MilwaukeeNational Science Foundation
KeywordsDissolved organic carbonBiogeochemical cycleChemistryEnvironmental chemistryAbsorbanceHumusOrganic matterArcticEnvironmental scienceOceanographyGeologyChromatographySoil scienceOrganic chemistry

Abstract

fetched live from OpenAlex

Abstract Arctic rivers are sensitive to climate and environmental change, but the biogeochemical response remains poorly understood. Monthly size‐fractionated dissolved organic matter (DOM) samples from the lower Yukon River were characterized using UV–visible, fluorescence, and Fourier transform‐infrared (FT‐IR) spectroscopy techniques. The EEM‐PARAFAC analysis revealed three major fluorescent DOM components, including two humic‐like components (C 480 and C 400 ) and one protein‐like component (C 310 ), with their relative importance following the order of C 480 ≥ C 400 > C 310 in the high‐molecular‐weight DOM (1 kDa–0.4 μ m) and C 400 > C 480 > C 310 in the low‐molecular‐weight DOM pool (< 1 kDa). Transformation in DOM and change in sources were manifested in major fluorescent components and optical properties, including biological index (BIX), humification index (HIX), spectral slope ( S 275–295 ) and specific UV absorbance at 254 nm (SUVA 254 ). These changes occurred within different DOM size‐fractions and among ice‐covered, spring freshet, and open seasons. Joint analysis of EEM and FT‐IR spectra using a data fusion technique showed that humic‐like DOM is mostly associated with C─H, C═C, and C─O bonds, while protein‐like DOM is correlated more with C─N and N─H related structures. DOM aromaticity and the ratios of HIX to BIX and protein‐like to humic‐like components may be used as a compelling proxy to measure change in source waters and to infer permafrost dynamics. Our results provide insight into the seasonal variation in DOM composition for different size‐fractions in the lower Yukon River, and a baseline dataset against which future changes can be understood in the context of arctic basin biogeochemical cycling.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame machine prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. The Gemma side is a direct model label for every work in the frame, read from the title-only record. The Codex side is a classifier learned from the 10,348 direct Codex labels and calibrated to design-weighted sample rates; fields without enough sample support carry no Codex call. Candidate is the union of the two sides; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: metacan-v3-hybrid-931329e0061cValidation status: machine_predicted_unvalidated
Candidate categoriesnone
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Observational · Consensus signal: Observational
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.036
Threshold uncertainty score0.071

Distilled classifier scores by category (both heads)

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0000.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.000
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0000.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.004
GPT teacher head0.181
Teacher spread0.177 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one source (direct Gemma or distilled Codex), not a consensus.

The models applied no category: nothing in the taxonomy fit this work.
Study designObservational
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations40
Published2021
Admission routes2
Has abstractyes

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