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Record W3187822831 · doi:10.1021/acsapm.1c00640

Environmentally Friendly and Zero-Formamide EVA/LDPE Microcellular Foams via Supercritical Carbon Dioxide Solid Foaming

2021· article· en· W3187822831 on OpenAlex

Why this work is in the frame

A frame that forgets how it found something cannot be audited. These are the routes that admitted this work.

affAt least one author lists a Canadian institution in the pinned OpenAlex snapshot.

Bibliographic record

VenueACS Applied Polymer Materials · 2021
Typearticle
Languageen
FieldMaterials Science
TopicPolymer Foaming and Composites
Canadian institutionsUniversity of Toronto
FundersState Key Laboratory of Polymer Materials EngineeringSichuan UniversityNational Natural Science Foundation of China
KeywordsPolyolefinMaterials scienceLow-density polyethyleneComposite materialElastomerPolyethyleneSupercritical fluidUltimate tensile strengthBlowing agentSupercritical carbon dioxidePolyurethaneOrganic chemistry

Abstract

fetched live from OpenAlex

Elastomeric polyolefin foams with excellent mechanical properties, environmentally friendly performance, and cost effectiveness are highly promising. Nevertheless, it is a huge challenge to obtain these advantages in elastomeric polyolefin foams using chemical or common physical blowing agents. Therefore, a strategy was applied to the ethylene–vinyl acetate copolymer (EVA)/low-density polyethylene (LDPE) (EVA/LDPE) system by combining crosslinking, microphase separation, crystallization, and supercritical CO2 (scCO2) solid foaming. Consequently, environmentally friendly EVA/LDPE foams of zero formamide with the desired uniform cellular structure of expansion ratio over 8, average cell size less than 50 μm, and cell density over 109 #/cm3 were obtained. The lightweight EVA/LDPE foams show excellent tensile strength and compression strength, much higher than those of other elastomeric polyolefin foams. The reasons for this are that (1) the introduction of crosslinking and entanglement structures in EVA enhances the viscoelasticity, which is beneficial to bubble nucleation and bubble stability in the foam, and simultaneously improves the mechanical properties of the foam; (2) the existence of LDPE segments in EVA leads to microphase separation, which is beneficial to bubble nucleation; (3) low-temperature solid foaming enhances the mechanical properties of the foam due to the uniform microcellular structure; and (4) scCO2 foaming has zero formamide, which meets the safety requirements and specifications of children’s floor mats (T/CTJPA 005-2018).

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.000
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Bench or experimental · Consensus signal: Bench or experimental
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.006
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0000.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.000
Bibliometrics0.0000.000
Science and technology studies0.0000.000
Scholarly communication0.0000.000
Open science0.0000.001
Research integrity0.0000.000
Insufficient payload (model declined to judge)0.0010.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.005
GPT teacher head0.205
Teacher spread0.200 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it