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Record W3199037945

A Modelling Study of the Impact of Photolysis on Indoor Air Quality

2021· dissertation· en· W3199037945 on OpenAlexfundno aff
Zixu Wang

Bibliographic record

VenueWhite Rose Research Online (University of Leeds, The University of Sheffield, University of York) · 2021
Typedissertation
Languageen
FieldEnvironmental Science
TopicImpact of Light on Environment and Health
Canadian institutionsnot available
FundersCanada Research ChairsUniversity of LeedsAlfred P. Sloan Foundation
KeywordsRadicalPhotodissociationPeroxyacetyl nitrateHydroxyl radicalOzoneChemistryPhotochemistryEnvironmental chemistryNitrogen dioxideEnvironmental scienceIndoor air qualityPollutantCombustionMeteorologyNOxEnvironmental engineeringOrganic chemistry
DOInot available

Abstract

fetched live from OpenAlex

Most human exposure to air pollutants happen indoors, where people spend most of their time (~90%). In the ambient atmosphere, photolysis plays a major role in initiating chemical reactions. However, indoor photolysis is less well studied. Consequently, the role that photolysis plays in indoor chemical processing, particularly in the formation of harmful species, is unclear. The major aim of this thesis was, therefore, to improve the representation of indoor lighting and attenuated sunlight in the Indoor Detailed Chemical Model (INDCM). The improved model was then used to investigate the impacts of glass type, indoor artificial light, cloudiness, time of year and latitude on indoor photolysis rates and hence indoor air chemistry. 
\nThe results show that variations in glass composition produce the highest deviations (~71%) in predicted concentrations of key indoor species (ozone, nitrous acid, nitric oxide, hydroxyl radicals, hydroperoxy radicals, organic peroxy radicals, peroxyacetyl nitrates and organic nitrates), followed by cloud level (~53%) and proximity to artificial light source (~53%), when compared to baseline conditions. These impacts were greatest for predicted hydroxyl radical concentrations, which deviated by an average of ~142% from the baseline scenario depending on the conditions studied. 
\nEnhanced radical concentrations were found during two cleaning case studies (automated and traditional techniques), with predicted hydroxyl radical concentrations up to 1.3 × 107 and 1.5106 molecule/cm3 respectively. Furthermore, radical concentrations were found to be highest under stronger lighting conditions, persisting for several hours after the cleaning events.
\nThis study provides a valuable contribution to the understanding of the impacts of photolysis on indoor air chemistry. Indoor artificial lights, such as LED, together with low cut-off wavelength glasses, will likely reduce the effects of photolysis indoors, but more research is needed on the health effects of different indoor air mixtures to confirm this recommendation.

Fetched live from OpenAlex and de-inverted. Abstracts are not stored in this database: the inverted indexes are 8.6 GB of the frame’s 9.3 GB of text, and the host has 13 GB free.

How this classification was reachedexpand

Full frame distilled prediction

Teacher imitation

Not calibrated prevalence, not ground truth. Human validation pending. Learned from the 10,348 direct Codex labels and 10,348 direct Gemma labels. Candidate is the union of thresholded teacher heads; consensus is their intersection. These outputs are machine_predicted_unvalidated and are not human labels or direct frontier model labels.

metaresearch head score (Codex)0.002
metaresearch head score (Gemma)0.000
Version: codex-gemma-dda1882f352aValidation status: machine_predicted_unvalidated
Candidate categoriesMeta-epidemiology (narrow), Insufficient payload (model declined to judge)
Consensus categoriesnone
DomainCandidate signal: none · Consensus signal: none
Study designCandidate signal: Qualitative · Consensus signal: Qualitative
GenreCandidate signal: Empirical · Consensus signal: Empirical
Teacher disagreement score0.221
Threshold uncertainty score1.000

Codex and Gemma teacher scores by category

CategoryCodexGemma
Metaresearch0.0020.000
Meta-epidemiology (narrow)0.0000.000
Meta-epidemiology (broad)0.0010.001
Bibliometrics0.0010.001
Science and technology studies0.0010.002
Scholarly communication0.0000.000
Open science0.0030.001
Research integrity0.0000.001
Insufficient payload (model declined to judge)0.0030.000

Machine scores (provisional)

The two teacher heads of the student model, read on this work. A score orders the frame for review; it never asserts a category, and the validation status ships verbatim with every row.

Baseline scores from an immature model (maturity gate not passed, 7 training rounds). Scores rank; they never assert a category.

Opus teacher head0.061
GPT teacher head0.316
Teacher spread0.255 · how far apart the two teachers sit on this one work
Validation statusscore_only:v0-immature-baseline · verbatim from the scoring run: score_only means the number may rank works, and no category label ships from it

Classification

machine, unvalidated

Machine predicted; a candidate call from one teacher head, not a consensus.

Study designQualitative
Domainnot available
GenreEmpirical

How this classification was reached, model by model and score by score, is at the end of the page under "How this classification was reached".

Quick stats

Citations0
Published2021
Admission routes1
Has abstractyes

Explore more

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